Quantum oscillations

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Condensed matter
experiments
Levitation of a magnet on top of a superconductor 2.jpg
ARPES
ACAR
Neutron scattering
X-ray spectroscopy
Quantum oscillations
Scanning tunneling microscopy

In condensed matter physics, quantum oscillations describes a series of related experimental techniques used to map the Fermi surface of a metal in the presence of a strong magnetic field. [1] These techniques are based on the principle of Landau quantization of Fermions moving in a magnetic field. [2] For a gas of free fermions in a strong magnetic field, the energy levels are quantized into bands, called the Landau levels, whose separation is proportional to the strength of the magnetic field. In a quantum oscillation experiment, the external magnetic field is varied, which causes the Landau levels to pass over the Fermi surface, which in turn results in oscillations of the electronic density of states at the Fermi level; this produces oscillations in the many material properties which depend on this, including resistance (the Shubnikov–de Haas effect), Hall resistance, [2] and magnetic susceptibility (the de Haas–van Alphen effect). Observation of quantum oscillations in a material is considered a signature of Fermi liquid behaviour. [3]

Contents

Quantum oscillations have been used to study high temperature superconducting materials such as cuprates and pnictides. [1] Studies using these experiments have shown that the ground state of underdoped cuprates behave similar to a Fermi liquid, and display characteristics such as Landau quasiparticles. [4]

In 2021 this technique has been used to observe a predicted state called "electron–phonon fluid", [5] [6] a similar particle-quasiparticle state already known is the exciton–polariton fluid.

Experiment

When a magnetic field is applied to a system of free charged fermions, their energy states are quantized into the so-called Landau levels, given by [7]

YBCO superconductor under high magnetic field. As field strength is increased, superconductivity is suppressed and Landau oscillations can be observed Quantum oscillations at 100 T.jpg
YBCO superconductor under high magnetic field. As field strength is increased, superconductivity is suppressed and Landau oscillations can be observed

for integer-valued , where is the external magnetic field and are the fermion charge and effective mass respectively.

When the external magnetic field is increased in an isolated system, the Landau levels expand, and eventually "fall off" the Fermi surface. This leads to oscillations in the observed energy of the highest occupied level, and hence in many physical properties (including Hall conductivity, resistivity, and susceptibility). The periodicity of these oscillations can be measured, and in turn can be used to determine the cross-sectional area of the Fermi surface. [8] If the axis of the magnetic field is varied at constant magnitude, similar oscillations are observed. The oscillations occur whenever the Landau orbits touch the Fermi surface. In this way, the complete geometry of the Fermi sphere can be mapped. [8]

Underdoped cuprates

Studies of underdoped cuprate compounds such as YBa2Cu3O6+x through probes such as ARPES have indicated that these phases show characteristics of non-Fermi liquids, [9] and in particular, the absence of well-defined Landau quasiparticles. [10] However, quantum oscillations have been observed in these materials at low temperatures, if their superconductivity is suppressed by a sufficiently high magnetic field, [2] which is evidence for the presence of well-defined quasiparticles with fermionic statistics. These experimental results thus disagree with those from ARPES and other probes. [7]

See also

Related Research Articles

<span class="mw-page-title-main">Condensed matter physics</span> Branch of physics

Condensed matter physics is the field of physics that deals with the macroscopic and microscopic physical properties of matter, especially the solid and liquid phases that arise from electromagnetic forces between atoms and electrons. More generally, the subject deals with condensed phases of matter: systems of many constituents with strong interactions among them. More exotic condensed phases include the superconducting phase exhibited by certain materials at extremely low cryogenic temperatures, the ferromagnetic and antiferromagnetic phases of spins on crystal lattices of atoms, the Bose–Einstein condensates found in ultracold atomic systems, and liquid crystals. Condensed matter physicists seek to understand the behavior of these phases by experiments to measure various material properties, and by applying the physical laws of quantum mechanics, electromagnetism, statistical mechanics, and other physics theories to develop mathematical models and predict the properties of extremely large groups of atoms.

The quantum Hall effect is a quantized version of the Hall effect which is observed in two-dimensional electron systems subjected to low temperatures and strong magnetic fields, in which the Hall resistance Rxy exhibits steps that take on the quantized values

<span class="mw-page-title-main">Fermi liquid theory</span> Theoretical model in physics

Fermi liquid theory is a theoretical model of interacting fermions that describes the normal state of the conduction electrons in most metals at sufficiently low temperatures. The theory describes the behavior of many-body systems of particles in which the interactions between particles may be strong. The phenomenological theory of Fermi liquids was introduced by the Soviet physicist Lev Davidovich Landau in 1956, and later developed by Alexei Abrikosov and Isaak Khalatnikov using diagrammatic perturbation theory. The theory explains why some of the properties of an interacting fermion system are very similar to those of the ideal Fermi gas, and why other properties differ.

In condensed matter physics, a quasiparticle is a concept used to describe a collective behavior of a group of particles that can be treated as if they were a single particle. Formally, quasiparticles and collective excitations are closely related phenomena that arise when a microscopically complicated system such as a solid behaves as if it contained different weakly interacting particles in vacuum.

<span class="mw-page-title-main">Luttinger liquid</span> Theoretical model describing interacting fermions in a one-dimensional conductor

A Luttinger liquid, or Tomonaga–Luttinger liquid, is a theoretical model describing interacting electrons in a one-dimensional conductor. Such a model is necessary as the commonly used Fermi liquid model breaks down for one dimension.

In condensed matter physics, the Fermi surface is the surface in reciprocal space which separates occupied from unoccupied electron states at zero temperature. The shape of the Fermi surface is derived from the periodicity and symmetry of the crystalline lattice and from the occupation of electronic energy bands. The existence of a Fermi surface is a direct consequence of the Pauli exclusion principle, which allows a maximum of one electron per quantum state. The study of the Fermi surfaces of materials is called fermiology.

The fractional quantum Hall effect (FQHE) is a physical phenomenon in which the Hall conductance of 2-dimensional (2D) electrons shows precisely quantized plateaus at fractional values of , where e is the electron charge and h is the Planck constant. It is a property of a collective state in which electrons bind magnetic flux lines to make new quasiparticles, and excitations have a fractional elementary charge and possibly also fractional statistics. The 1998 Nobel Prize in Physics was awarded to Robert Laughlin, Horst Störmer, and Daniel Tsui "for their discovery of a new form of quantum fluid with fractionally charged excitations" The microscopic origin of the FQHE is a major research topic in condensed matter physics.

<span class="mw-page-title-main">Pseudogap</span> State at which a Fermi surface has a partial energy gap in condensed matter physics

In condensed matter physics, a pseudogap describes a state where the Fermi surface of a material possesses a partial energy gap, for example, a band structure state where the Fermi surface is gapped only at certain points.

<span class="mw-page-title-main">Type-II superconductor</span> Superconductor characterized by the formation of magnetic vortices in an applied magnetic field

In superconductivity, a type-II superconductor is a superconductor that exhibits an intermediate phase of mixed ordinary and superconducting properties at intermediate temperature and fields above the superconducting phases. It also features the formation of magnetic field vortices with an applied external magnetic field. This occurs above a certain critical field strength Hc1. The vortex density increases with increasing field strength. At a higher critical field Hc2, superconductivity is destroyed. Type-II superconductors do not exhibit a complete Meissner effect.

<span class="mw-page-title-main">Majorana fermion</span> Fermion that is its own antiparticle

A Majorana fermion, also referred to as a Majorana particle, is a fermion that is its own antiparticle. They were hypothesised by Ettore Majorana in 1937. The term is sometimes used in opposition to a Dirac fermion, which describes fermions that are not their own antiparticles.

The De Haas–Van Alphen effect, often abbreviated to DHVA, is a quantum mechanical effect in which the magnetic susceptibility of a pure metal crystal oscillates as the intensity of the magnetic field B is increased. It can be used to determine the Fermi surface of a material. Other quantities also oscillate, such as the electrical resistivity, specific heat, and sound attenuation and speed. It is named after Wander Johannes de Haas and his student Pieter M. van Alphen. The DHVA effect comes from the orbital motion of itinerant electrons in the material. An equivalent phenomenon at low magnetic fields is known as Landau diamagnetism.

An oscillation in the conductivity of a material that occurs at low temperatures in the presence of very intense magnetic fields, the Shubnikov–de Haas effect (SdH) is a macroscopic manifestation of the inherent quantum mechanical nature of matter. It is often used to determine the effective mass of charge carriers, allowing investigators to distinguish among majority and minority carrier populations. The effect is named after Wander Johannes de Haas and Lev Shubnikov.

In quantum mechanics, the energies of cyclotron orbits of charged particles in a uniform magnetic field are quantized to discrete values, called Landau levels. These levels are degenerate, with the number of electrons per level directly proportional to the strength of the applied magnetic field. It is named after the Soviet physicist Lev Landau.

<span class="mw-page-title-main">Angle-resolved photoemission spectroscopy</span> Experimental technique to determine the distribution of electrons in solids

Angle-resolved photoemission spectroscopy (ARPES) is an experimental technique used in condensed matter physics to probe the allowed energies and momenta of the electrons in a material, usually a crystalline solid. It is based on the photoelectric effect, in which an incoming photon of sufficient energy ejects an electron from the surface of a material. By directly measuring the kinetic energy and emission angle distributions of the emitted photoelectrons, the technique can map the electronic band structure and Fermi surfaces. ARPES is best suited for the study of one- or two-dimensional materials. It has been used by physicists to investigate high-temperature superconductors, graphene, topological materials, quantum well states, and materials exhibiting charge density waves.

In Materials Science, heavy fermion materials are a specific type of intermetallic compound, containing elements with 4f or 5f electrons in unfilled electron bands. Electrons are one type of fermion, and when they are found in such materials, they are sometimes referred to as heavy electrons. Heavy fermion materials have a low-temperature specific heat whose linear term is up to 1000 times larger than the value expected from the free electron model. The properties of the heavy fermion compounds often derive from the partly filled f-orbitals of rare-earth or actinide ions, which behave like localized magnetic moments.

<span class="mw-page-title-main">Subir Sachdev</span> Indian physicist

Subir Sachdev is Herchel Smith Professor of Physics at Harvard University specializing in condensed matter. He was elected to the U.S. National Academy of Sciences in 2014, received the Lars Onsager Prize from the American Physical Society and the Dirac Medal from the ICTP in 2018, and was elected Foreign Member of the Royal Society ForMemRS in 2023. He was a co-editor of the Annual Review of Condensed Matter Physics 2017–2019, and is Editor-in-Chief of Reports on Progress in Physics 2022-.

A composite fermion is the topological bound state of an electron and an even number of quantized vortices, sometimes visually pictured as the bound state of an electron and, attached, an even number of magnetic flux quanta. Composite fermions were originally envisioned in the context of the fractional quantum Hall effect, but subsequently took on a life of their own, exhibiting many other consequences and phenomena.

In the field of unconventional superconductivity, a Fermi arc is a phenomenon visible in the pseudogap state of a superconductor. Seen in momentum space, part of the space exhibits a gap in the density of states, like in a superconductor. This starts at the antinodal points, and spreads through momentum space when lowering the temperature until everywhere is gapped and the sample is superconducting. The area in momentum space that remains ungapped is called the Fermi arc.

The term Dirac matter refers to a class of condensed matter systems which can be effectively described by the Dirac equation. Even though the Dirac equation itself was formulated for fermions, the quasi-particles present within Dirac matter can be of any statistics. As a consequence, Dirac matter can be distinguished in fermionic, bosonic or anyonic Dirac matter. Prominent examples of Dirac matter are graphene and other Dirac semimetals, topological insulators, Weyl semimetals, various high-temperature superconductors with -wave pairing and liquid helium-3. The effective theory of such systems is classified by a specific choice of the Dirac mass, the Dirac velocity, the gamma matrices and the space-time curvature. The universal treatment of the class of Dirac matter in terms of an effective theory leads to a common features with respect to the density of states, the heat capacity and impurity scattering.

References

  1. 1 2 Coldea, Amalia (2010). "Quantum oscillations probe the normal electronic states of novel superconductors". Philosophical Transactions of the Royal Society A. 368 (1924): 3503–3517. Bibcode:2010RSPTA.368.3503C. doi: 10.1098/rsta.2010.0089 . PMID   20603364 . Retrieved 20 March 2012.
  2. 1 2 3 Doiron-Leyraud, Nicolas; et al. (2007). "Quantum oscillations and the Fermi surface in an underdoped high-Tc superconductor". Nature. 447 (7144): 565–8. arXiv: 0801.1281 . Bibcode:2007Natur.447..565D. doi:10.1038/nature05872. PMID   17538614. S2CID   4397560.
  3. Condensed-matter and materials physics: the science of the world around us. National Research Council. 2010. ISBN   978-0-309-13409-5.
  4. Broun, D. M. (2008). "What lies beneath the dome?". Nature Physics. 4 (3): 170–172. Bibcode:2008NatPh...4..170B. doi:10.1038/nphys909.
  5. Yang, Hung-Yu; Yao, Xiaohan; Plisson, Vincent; Mozaffari, Shirin; Scheifers, Jan P.; Savvidou, Aikaterini Flessa; Choi, Eun Sang; McCandless, Gregory T.; Padlewski, Mathieu F.; Putzke, Carsten; Moll, Philip J. W. (2021-09-06). "Evidence of a coupled electron-phonon liquid in NbGe2". Nature Communications. 12 (1): 5292. arXiv: 2103.01515 . Bibcode:2021NatCo..12.5292Y. doi:10.1038/s41467-021-25547-x. ISSN   2041-1723. PMC   8421384 . PMID   34489411.
  6. College, Boston (2021-09-06). "Novel Metal Discovered Where Electrons Flow in the Same Way Water Flows in a Pipe". SciTechDaily. Retrieved 2021-09-20.
  7. 1 2 Sebastian, Suchitra E.; Neil Harrison; Gilbert G. Lonzarich (2011). "Quantum oscillations in the high-Tc cuprates". Philosophical Transactions of the Royal Society A. 369 (1941): 1687–1711. Bibcode:2011RSPTA.369.1687S. doi: 10.1098/rsta.2010.0243 . PMID   21422021 . Retrieved 23 March 2012.
  8. 1 2 Ibach, Harald; Hans Lüth (1995). Solid-state physics: an introduction to principles of materials science. Berlin: Springer-Verlag. ISBN   978-3-540-58573-2.
  9. Alexandrov, A. S. (2008). "Theory of quantum magneto-oscillations in underdoped cuprate superconductors". Journal of Physics: Condensed Matter. 20 (19): 192202. arXiv: 0711.0093 . Bibcode:2008JPCM...20s2202A. doi:10.1088/0953-8984/20/19/192202. S2CID   117020227.
  10. Damascelli, Andrea; Hussain, Zahid; Zhi-Xun Shen (2003). "Angle-resolved photoemission studies of the cuprate superconductors". Reviews of Modern Physics. 75 (2): 473. arXiv: cond-mat/0208504 . Bibcode:2003RvMP...75..473D. doi:10.1103/RevModPhys.75.473. S2CID   118433150.