Neutron howitzer

Last updated May 23, 2024

A neutron howitzer is a neutron source that emits neutrons in a single direction. It was discovered in the 1930s that alpha radiation that strikes the beryllium nucleus would release neutrons. The high speed of the alpha is sufficient to overcome the relatively low Coulomb barrier of the beryllium nucleus, the repulsive force due to the positive charge of the nucleus, which contains only four protons, allowing for fusion of the two particles, releasing energetic neutrons.

In 1930 Walther Bothe and Herbert Becker in Germany found that alpha particles striking light elements such as beryllium, boron, or lithium would release a highly penetrating radiation, at first believed to be gamma radiation, although it was more penetrating than any gamma rays known. The next important contribution was reported in 1932 by Irène Joliot-Curie and Frédéric Joliot in Paris, who showed that if this unknown radiation fell on paraffin wax or any other hydrogen-containing compound it ejected protons of very high energy. Finally, in 1932 the physicist James Chadwick in England performed a series of experiments showing that the gamma ray hypothesis was untenable, and suggested that the new radiation consisted of uncharged particles of approximately the mass of the proton. He performed a series of experiments to verify this, these uncharged particles were eventually called "neutrons", and Chadwick is credited with this discovery.

Any alpha-emitting radioisotope will suffice, but usually a high specific activity alpha-emitter is chosen. Historically a variety of isotopes such as radium (Ra-226) were used, but in modern times the transuranic isotopes Am-241 and Pu-239 are almost exclusively used in AmBe and PuBe neutron sources, respectively.^[1] The alpha emitter and the beryllium are pulverized and mixed together in close intimate contact to ensure a high percentage of alpha-emitter and beryllium nuclei in close contact, since the alpha particle has a very short range through material, and would lose energy preventing reaction if sufficiently far away. This mixture of material is then packed into a suitable carrier with radiation shielding, with one end open to allow the neutrons to shoot out in the direction of the open end, thus acting like a howitzer.^[2]^[3]^[4]

Neutron howitzers were used by Otto Hahn, Fritz Strassman, and Lise Meitner in 1938 to bombard uranium nuclei with neutrons in the hopes of making transuranic elements. To their surprise, they found barium residue, a clear indication that they had instead fissioned uranium nuclei. This discovery led to the development of the first nuclear reactor in 1942, and ultimately nuclear weapons in 1945.

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Atoms are the basic particles of the chemical elements. An atom consists of a nucleus of protons and generally neutrons, surrounded by an electromagnetically bound swarm of electrons. The chemical elements are distinguished from each other by the number of protons that are in their atoms. For example, any atom that contains 11 protons is sodium, and any atom that contains 29 protons is copper. Atoms with the same number of protons but a different number of neutrons are called isotopes of the same element.

Alpha decay or α-decay is a type of radioactive decay in which an atomic nucleus emits an alpha particle and thereby transforms or "decays" into a different atomic nucleus, with a mass number that is reduced by four and an atomic number that is reduced by two. An alpha particle is identical to the nucleus of a helium-4 atom, which consists of two protons and two neutrons. It has a charge of +2 e and a mass of 4 Da. For example, uranium-238 decays to form thorium-234.

The neutron is a subatomic particle, symbol n or n⁰
, which has a neutral charge, and a mass slightly greater than that of a proton. Protons and neutrons constitute the nuclei of atoms. Since protons and neutrons behave similarly within the nucleus, they are both referred to as nucleons. Nucleons have a mass of approximately one atomic mass unit, or dalton. Their properties and interactions are described by nuclear physics. Protons and neutrons are not elementary particles; each is composed of three quarks.

<span class="mw-page-title-main">Nuclear physics</span> Field of physics that studies atomic nuclei

Nuclear physics is the field of physics that studies atomic nuclei and their constituents and interactions, in addition to the study of other forms of nuclear matter.

Neutron activation analysis (NAA) is a nuclear process used for determining the concentrations of elements in many materials. NAA allows discrete sampling of elements as it disregards the chemical form of a sample, and focuses solely on atomic nuclei. The method is based on neutron activation and thus requires a neutron source. The sample is bombarded with neutrons, causing its constituent elements to form radioactive isotopes. The radioactive emissions and radioactive decay paths for each element have long been studied and determined. Using this information, it is possible to study spectra of the emissions of the radioactive sample, and determine the concentrations of the various elements within it. A particular advantage of this technique is that it does not destroy the sample, and thus has been used for the analysis of works of art and historical artifacts. NAA can also be used to determine the activity of a radioactive sample.

Nuclear fission is a reaction in which the nucleus of an atom splits into two or more smaller nuclei. The fission process often produces gamma photons, and releases a very large amount of energy even by the energetic standards of radioactive decay.

In physics, radiation is the emission or transmission of energy in the form of waves or particles through space or a material medium. This includes:

A beta particle, also called beta ray or beta radiation, is a high-energy, high-speed electron or positron emitted by the radioactive decay of an atomic nucleus during the process of beta decay. There are two forms of beta decay, β⁻ decay and β⁺ decay, which produce electrons and positrons respectively.

A neutron source is any device that emits neutrons, irrespective of the mechanism used to produce the neutrons. Neutron sources are used in physics, engineering, medicine, nuclear weapons, petroleum exploration, biology, chemistry, and nuclear power. Neutron source variables include the energy of the neutrons emitted by the source, the rate of neutrons emitted by the source, the size of the source, the cost of owning and maintaining the source, and government regulations related to the source.

Ionizing radiation (US) (or ionising radiation [UK]), including nuclear radiation, consists of subatomic particles or electromagnetic waves that have sufficient energy to ionize atoms or molecules by detaching electrons from them. Some particles can travel up to 99% of the speed of light, and the electromagnetic waves are on the high-energy portion of the electromagnetic spectrum.

Neutron radiation is a form of ionizing radiation that presents as free neutrons. Typical phenomena are nuclear fission or nuclear fusion causing the release of free neutrons, which then react with nuclei of other atoms to form new nuclides—which, in turn, may trigger further neutron radiation. Free neutrons are unstable, decaying into a proton, an electron, plus an electron antineutrino. Free neutrons have a mean lifetime of 887 seconds.

<span class="mw-page-title-main">Uranium-238</span> Isotope of uranium

Uranium-238 is the most common isotope of uranium found in nature, with a relative abundance of 99%. Unlike uranium-235, it is non-fissile, which means it cannot sustain a chain reaction in a thermal-neutron reactor. However, it is fissionable by fast neutrons, and is fertile, meaning it can be transmuted to fissile plutonium-239. ²³⁸U cannot support a chain reaction because inelastic scattering reduces neutron energy below the range where fast fission of one or more next-generation nuclei is probable. Doppler broadening of ²³⁸U's neutron absorption resonances, increasing absorption as fuel temperature increases, is also an essential negative feedback mechanism for reactor control.

Neutron capture is a nuclear reaction in which an atomic nucleus and one or more neutrons collide and merge to form a heavier nucleus. Since neutrons have no electric charge, they can enter a nucleus more easily than positively charged protons, which are repelled electrostatically.

<span class="mw-page-title-main">Nuclear binding energy</span> Minimum energy required to separate particles within a nucleus

Nuclear binding energy in experimental physics is the minimum energy that is required to disassemble the nucleus of an atom into its constituent protons and neutrons, known collectively as nucleons. The binding energy for stable nuclei is always a positive number, as the nucleus must gain energy for the nucleons to move apart from each other. Nucleons are attracted to each other by the strong nuclear force. In theoretical nuclear physics, the nuclear binding energy is considered a negative number. In this context it represents the energy of the nucleus relative to the energy of the constituent nucleons when they are infinitely far apart. Both the experimental and theoretical views are equivalent, with slightly different emphasis on what the binding energy means.

Induced radioactivity, also called artificial radioactivity or man-made radioactivity, is the process of using radiation to make a previously stable material radioactive. The husband-and-wife team of Irène Joliot-Curie and Frédéric Joliot-Curie discovered induced radioactivity in 1934, and they shared the 1935 Nobel Prize in Chemistry for this discovery.

<span class="mw-page-title-main">Valley of stability</span> Characterization of nuclide stability

In nuclear physics, the valley of stability is a characterization of the stability of nuclides to radioactivity based on their binding energy. Nuclides are composed of protons and neutrons. The shape of the valley refers to the profile of binding energy as a function of the numbers of neutrons and protons, with the lowest part of the valley corresponding to the region of most stable nuclei. The line of stable nuclides down the center of the valley of stability is known as the line of beta stability. The sides of the valley correspond to increasing instability to beta decay. The decay of a nuclide becomes more energetically favorable the further it is from the line of beta stability. The boundaries of the valley correspond to the nuclear drip lines, where nuclides become so unstable they emit single protons or single neutrons. Regions of instability within the valley at high atomic number also include radioactive decay by alpha radiation or spontaneous fission. The shape of the valley is roughly an elongated paraboloid corresponding to the nuclide binding energies as a function of neutron and atomic numbers.

Photodisintegration is a nuclear process in which an atomic nucleus absorbs a high-energy gamma ray, enters an excited state, and immediately decays by emitting a subatomic particle. The incoming gamma ray effectively knocks one or more neutrons, protons, or an alpha particle out of the nucleus. The reactions are called (γ,n), (γ,p), and (γ,α).

Alpha particles, also called alpha rays or alpha radiation, consist of two protons and two neutrons bound together into a particle identical to a helium-4 nucleus. They are generally produced in the process of alpha decay but may also be produced in other ways. Alpha particles are named after the first letter in the Greek alphabet, α. The symbol for the alpha particle is α or α²⁺. Because they are identical to helium nuclei, they are also sometimes written as He²⁺
or ⁴
₂He²⁺
indicating a helium ion with a +2 charge. Once the ion gains electrons from its environment, the alpha particle becomes a normal helium atom ⁴
₂He.

<span class="mw-page-title-main">Discovery of the neutron</span> Scientific background leading to the discovery of subatomic particles

The discovery of the neutron and its properties was central to the extraordinary developments in atomic physics in the first half of the 20th century. Early in the century, Ernest Rutherford developed a crude model of the atom, based on the gold foil experiment of Hans Geiger and Ernest Marsden. In this model, atoms had their mass and positive electric charge concentrated in a very small nucleus. By 1920, isotopes of chemical elements had been discovered, the atomic masses had been determined to be (approximately) integer multiples of the mass of the hydrogen atom, and the atomic number had been identified as the charge on the nucleus. Throughout the 1920s, the nucleus was viewed as composed of combinations of protons and electrons, the two elementary particles known at the time, but that model presented several experimental and theoretical contradictions.

Nuclear fission was discovered in December 1938 by chemists Otto Hahn and Fritz Strassmann and physicists Lise Meitner and Otto Robert Frisch. Fission is a nuclear reaction or radioactive decay process in which the nucleus of an atom splits into two or more smaller, lighter nuclei and often other particles. The fission process often produces gamma rays and releases a very large amount of energy, even by the energetic standards of radioactive decay. Scientists already knew about alpha decay and beta decay, but fission assumed great importance because the discovery that a nuclear chain reaction was possible led to the development of nuclear power and nuclear weapons. Hahn was awarded the 1944 Nobel Prize in Chemistry for the discovery of nuclear fission.

References

↑ Vega-Carillo, Héctor René; Manzanares-Acuña, Eduardo; Becerra-Ferreiro, Ana Maria; Carillo-Nuñez, Aureliano (2002). "Neutron and gamma-ray spectra of ²³⁹PuBe and ²⁴¹AmBe". Applied Radiation and Isotopes. 57 (2): 167–170. doi:10.1016/S0969-8043(02)00083-0. PMID 12150274.
↑ Cox, A.J.; Francois, P.E.; Gatrell, R.P. (1968). "The design of neutron howitzers". The International Journal of Applied Radiation and Isotopes. 19 (6): 541–4. doi:10.1016/0020-708X(68)90009-4.
↑ Jha, D. K. (2004). Elements of Nuclear Reactors. ISBN 9788171418831.
↑ "Oregon Administrative Rules". 2001.

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[1] Vega-Carillo, Héctor René; Manzanares-Acuña, Eduardo; Becerra-Ferreiro, Ana Maria; Carillo-Nuñez, Aureliano (2002). "Neutron and gamma-ray spectra of ²³⁹PuBe and ²⁴¹AmBe". Applied Radiation and Isotopes. 57 (2): 167–170. doi:10.1016/S0969-8043(02)00083-0. PMID 12150274.

[2] Cox, A.J.; Francois, P.E.; Gatrell, R.P. (1968). "The design of neutron howitzers". The International Journal of Applied Radiation and Isotopes. 19 (6): 541–4. doi:10.1016/0020-708X(68)90009-4.

[3] Jha, D. K. (2004). Elements of Nuclear Reactors. ISBN 9788171418831.

[4] "Oregon Administrative Rules". 2001.

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