Nuclear data

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Nuclear data represents measured (or evaluated) probabilities of various physical interactions involving the nuclei of atoms. It is used to understand the nature of such interactions by providing the fundamental input to many models and simulations, such as fission and fusion reactor calculations, shielding and radiation protection calculations, criticality safety, nuclear weapons, nuclear physics research, medical radiotherapy, radioisotope therapy and diagnostics, particle accelerator design and operations, geological and environmental work, radioactive waste disposal calculations, and space travel calculations.

Contents

It groups all experimental data relevant for nuclear physics and nuclear engineering. It includes a large number of physical quantities, like scattering and reaction cross sections (which are generally functions of energy and angle), nuclear structure and nuclear decay parameters, etc. It can involve neutrons, protons, deuterons, alpha particles, and virtually all nuclear isotopes which can be handled in a laboratory.

There are two major reasons to need high-quality nuclear data: theoretical model development of nuclear physics, and applications involving radiation and nuclear power. There is often an interplay between these two aspects, since applications often motivate research in particular theoretical fields, and theory can be used to predict quantities or phenomena which can lead to new or improved technological concepts. [1]

Nuclear Data Evaluations

To ensure a level of quality required to protect the public, experimental nuclear data results are occasionally evaluated by a Nuclear Data Organization to form a nuclear data library. These organizations review multiple measurements and agree upon the highest-quality measurements before publishing the libraries. For unmeasured or very complex data regimes, the parameters of nuclear models are adjusted until the resulting data matches well with critical experiments. The result of an evaluation is almost universally stored as a set of data files in Evaluated Nuclear Data File (ENDF) format. To keep the size of these files reasonable, they contain a combination of actual data tables and resonance parameters that can be reconstructed into pointwise data with specialized tools (such as NJOY).

Nuclear Data Organizations

Releases of ENDF/B Files

The historical releases of ENDF/B files are summarized below.

File versionRelease Date [2]
ENDF/B-I1968
ENDF/B-II1970
ENDF/B-III1972
ENDF/B-IV1974
ENDF/B-V1978
ENDF/B-VI1990
ENDF/B-VII2006
ENDF/B-VII.12011 [3]
ENDF/B-VIII2018 [4]

The historical releases of JEFF files are summarized below.

File versionRelease Date [5]
JEF-2.21992
JEFF-3.02002
JEFF-3.12005
JEFF-3.1.12009
JEFF-3.1.22011
JEFF-3.22014
JEFF-3.32017

See also

Related Research Articles

<span class="mw-page-title-main">Nuclear fusion</span> Process of combining atomic nuclei

Nuclear fusion is a reaction in which two or more atomic nuclei, usually deuterium and tritium, combine to form one or more different atomic nuclei and subatomic particles. The difference in mass between the reactants and products is manifested as either the release or absorption of energy. This difference in mass arises due to the difference in nuclear binding energy between the atomic nuclei before and after the reaction. Nuclear fusion is the process that powers active or main-sequence stars and other high-magnitude stars, where large amounts of energy are released.

<span class="mw-page-title-main">Neutron cross section</span> Measure of neutron interaction likelihood

In nuclear physics, the concept of a neutron cross section is used to express the likelihood of interaction between an incident neutron and a target nucleus. The neutron cross section σ can be defined as the area in cm2 for which the number of neutron-nuclei reactions taking place is equal to the product of the number of incident neutrons that would pass through the area and the number of target nuclei. In conjunction with the neutron flux, it enables the calculation of the reaction rate, for example to derive the thermal power of a nuclear power plant. The standard unit for measuring the cross section is the barn, which is equal to 10−28 m2 or 10−24 cm2. The larger the neutron cross section, the more likely a neutron will react with the nucleus.

Monte Carlo N-Particle Transport (MCNP) is a general-purpose, continuous-energy, generalized-geometry, time-dependent, Monte Carlo radiation transport code designed to track many particle types over broad ranges of energies and is developed by Los Alamos National Laboratory. Specific areas of application include, but are not limited to, radiation protection and dosimetry, radiation shielding, radiography, medical physics, nuclear criticality safety, detector design and analysis, nuclear oil well logging, accelerator target design, fission and fusion reactor design, decontamination and decommissioning. The code treats an arbitrary three-dimensional configuration of materials in geometric cells bounded by first- and second-degree surfaces and fourth-degree elliptical tori.

Caesium (55Cs) has 41 known isotopes, the atomic masses of these isotopes range from 112 to 152. Only one isotope, 133Cs, is stable. The longest-lived radioisotopes are 135Cs with a half-life of 1.33 million years, 137
Cs
with a half-life of 30.1671 years and 134Cs with a half-life of 2.0652 years. All other isotopes have half-lives less than 2 weeks, most under an hour.

Tin (50Sn) is the element with the greatest number of stable isotopes. This is probably related to the fact that 50 is a "magic number" of protons. In addition, twenty-nine unstable tin isotopes are known, including tin-100 (100Sn) and tin-132 (132Sn), which are both "doubly magic". The longest-lived tin radioisotope is tin-126 (126Sn), with a half-life of 230,000 years. The other 28 radioisotopes have half-lives of less than a year.

Naturally occurring zirconium (40Zr) is composed of four stable isotopes (of which one may in the future be found radioactive), and one very long-lived radioisotope (96Zr), a primordial nuclide that decays via double beta decay with an observed half-life of 2.0×1019 years; it can also undergo single beta decay, which is not yet observed, but the theoretically predicted value of t1/2 is 2.4×1020 years. The second most stable radioisotope is 93Zr, which has a half-life of 1.53 million years. Thirty other radioisotopes have been observed. All have half-lives less than a day except for 95Zr (64.02 days), 88Zr (83.4 days), and 89Zr (78.41 hours). The primary decay mode is electron capture for isotopes lighter than 92Zr, and the primary mode for heavier isotopes is beta decay.

Plutonium (94Pu) is an artificial element, except for trace quantities resulting from neutron capture by uranium, and thus a standard atomic weight cannot be given. Like all artificial elements, it has no stable isotopes. It was synthesized long before being found in nature, the first isotope synthesized being plutonium-238 in 1940. Twenty plutonium radioisotopes have been characterized. The most stable are plutonium-244 with a half-life of 80.8 million years, plutonium-242 with a half-life of 373,300 years, and plutonium-239 with a half-life of 24,110 years. All of the remaining radioactive isotopes have half-lives that are less than 7,000 years. This element also has eight meta states; all have half-lives of less than one second.

Bohrium (107Bh) is an artificial element. Like all artificial elements, it has no stable isotopes, and a standard atomic weight cannot be given. The first isotope to be synthesized was 262Bh in 1981. There are 11 known isotopes ranging from 260Bh to 274Bh, and 1 isomer, 262mBh. The longest-lived isotope is 270Bh with a half-life of 2.4 minutes, although the unconfirmed 278Bh may have an even longer half-life of about 690 seconds.

Hassium (108Hs) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 265Hs in 1984. There are 13 known isotopes from 263Hs to 277Hs and 1–4 isomers. The most stable isotope of hassium cannot be determined based on existing data due to uncertainty that arises from the low number of measurements. The half-lives of 269Hs and 271Hs are about 12 seconds, whereas that of 270Hs is about 7.6 seconds. It is also possible that 277mHs is more stable than these, with its half-life likely being 130±100 seconds, but only one event of decay of this isotope has been registered as of 2016.

Meitnerium (109Mt) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 266Mt in 1982, and this is also the only isotope directly synthesized; all other isotopes are only known as decay products of heavier elements. There are eight known isotopes, from 266Mt to 278Mt. There may also be two isomers. The longest-lived of the known isotopes is 278Mt with a half-life of 8 seconds. The unconfirmed heavier 282Mt appears to have an even longer half-life of 67 seconds.

Darmstadtium (110Ds) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 269Ds in 1994. There are 11 known radioisotopes from 267Ds to 281Ds and 2 or 3 known isomers. The longest-lived isotope is 281Ds with a half-life of 14 seconds.

Roentgenium (111Rg) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 272Rg in 1994, which is also the only directly synthesized isotope; all others are decay products of heavier elements. There are seven known radioisotopes, having mass numbers of 272, 274, and 278–282. The longest-lived isotope is 282Rg with a half-life of about 2 minutes, although the unconfirmed 283Rg and 286Rg may have longer half-lives of about 5.1 minutes and 10.7 minutes respectively.

Copernicium (112Cn) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 277Cn in 1996. There are 6 known radioisotopes ; the longest-lived isotope is 285Cn with a half-life of 30 seconds.

Nihonium (113Nh) is a synthetic element. Being synthetic, a standard atomic weight cannot be given and like all artificial elements, it has no stable isotopes. The first isotope to be synthesized was 284Nh as a decay product of 288Mc in 2003. The first isotope to be directly synthesized was 278Nh in 2004. There are 6 known radioisotopes from 278Nh to 286Nh, along with the unconfirmed 287Nh and 290Nh. The longest-lived isotope is 286Nh with a half-life of 9.5 seconds.

Flerovium (114Fl) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no stable isotopes. The first isotope to be synthesized was 289Fl in 1999. Flerovium has six known isotopes, along with the unconfirmed 290Fl, and possibly two nuclear isomers. The longest-lived isotope is 289Fl with a half-life of 1.9 seconds, but 290Fl may have a longer half-life of 19 seconds.

Moscovium (115Mc) is a synthetic element, and thus a standard atomic weight cannot be given. Like all synthetic elements, it has no known stable isotopes. The first isotope to be synthesized was 288Mc in 2004. There are five known radioisotopes from 286Mc to 290Mc. The longest-lived isotope is 290Mc with a half-life of 0.65 seconds.

Livermorium (116Lv) is an artificial element, and thus a standard atomic weight cannot be given. Like all artificial elements, it has no stable isotopes. The first isotope to be synthesized was 293Lv in 2000. There are five known radioisotopes, with mass numbers 288 and 290–293, as well as a few suggestive indications of a possible heavier isotope 294Lv. The longest-lived known isotope is 293Lv with a half-life of 70 ms.

<span class="mw-page-title-main">LISE++</span>

The program LISE++ is designed to predict the intensity and purity of radioactive ion beams (RIB) produced by In-flight separators. LISE++ also facilitates the tuning of experiments where its results can be quickly compared to on-line data. The program is constantly expanding and evolving from the feedback of its users around the world.

The National Nuclear Data Center is an organization based in the Brookhaven National Laboratory that acts as a repository for data regarding nuclear chemistry, such as nuclear structure, decay, and reaction data, as well as historical information regarding previous experiments and literature. According to the ResearchGATE scientific network, "The National Nuclear Data Center NNDC collects, evaluates, and disseminates nuclear physics data for basic nuclear research and applied nuclear technologies." The current Center Head is Dr. David Brown.

Unbiunium, also known as eka-actinium or element 121, is a hypothetical chemical element; it has symbol Ubu and atomic number 121. Unbiunium and Ubu are the temporary systematic IUPAC name and symbol respectively, which are used until the element is discovered, confirmed, and a permanent name is decided upon. In the periodic table of the elements, it is expected to be the first of the superactinides, and the third element in the eighth period. It has attracted attention because of some predictions that it may be in the island of stability. It is also likely to be the first of a new g-block of elements.

References

  1. Aliberti, G.; Palmiotti, G.; Salvatores, M.; Kim, T.K.; Taiwo, T.A.; Anitescu, M.; Kodeli, I.; Sartori, E.; Bosq, J.C.; Tommasi, J. (2006). "Nuclear data sensitivity, uncertainty and target accuracy assessment for future nuclear systems" (PDF). Annals of Nuclear Energy. 33 (8): 700–733. doi:10.1016/j.anucene.2006.02.003 . Retrieved 2018-06-07.
  2. Oblozinsky, Pavel (August 10, 2006). "Nuclear Data: New ENDF/B-VII Library" (PDF). Brookhaven National Laboratory. Retrieved 2014-07-01.
  3. Oblozinsky, Pavel (December 2011). "Special Issue on ENDF/B-VII.1 Library". Nuclear Data Sheets.
  4. Brown, David (February 2, 2018). "ENDF/B-VIII.0". Cross Section Evaluation Working Group (CSEWG) Announcement, Brookhaven National Laboratory. Retrieved 2018-02-19.
  5. "NEA JEFF page" . Retrieved 2019-08-12.