International Noble Gas Experiment

Last updated

The International Noble Gas Experiment (INGE) was formed in 1999 as an informal expert's group of developers of radioactive xenon measurement systems for the International Monitoring System for the Comprehensive Nuclear-Test-Ban Treaty (CTBT) (signed in 1997, but which has not entered into force). The group originally consisted of research and development groups from Germany, France, Russia, Sweden, and the United States, as well as personnel from Provisional Technical Secretariat of the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization CTBTO.

Contents

The INGE group was formed to test aspects of measuring xenon fission product radionuclides released by nuclear explosions. The systems developed and participating in the INGE measure xenon isotopes in the atmosphere and includes 131mXe, 133Xe, 133mXe, and 135Xe.

Since the INGE was formed in 1999, the group has expanded somewhat and now includes R&D and operational groups from many locations around the world. Although there is no official list of INGE members, the group is informally composed of scientists, engineers, and others from Argentina, Austria, Australia, Canada, China, France, Germany, Japan, Norway, South Korea, Sweden, Russia, the United States, and several other countries. These members regularly contribute to better understanding radioactive xenon measurements through operation of samplers, measurements of background at various locations, creation of data analysis routines, etc.

Staff from the preparatory commission of the CTBTO oversaw the experiment, with technical assistance from a German group of noble gas experts from the BfS in Freiburg, Germany. As of 2009, the experiment was still on-going, and so far it had consisted of 3 phases:

INGE Phase 1

The first phase of the INGE experiment took place in the laboratories. Four systems were developed to the point that they could measure xenon concentrations to specifications laid out by the CTBTO Preparatory Commission.

INGE Phase 2

The second phase of the INGE experiment took place in Freiburg, Germany, a location far away from the developers laboratories.

CountryInstituteRoleSystem Name
Germany(IAR) BfS System TesterN/A
France CEA/DASESystem DeveloperSPALAX
Russia KRI System DeveloperARIX
Sweden FOA (FOI) System DeveloperSAUNA Archived 2008-06-03 at the Wayback Machine
United States DOE/PNNL System Developer ARSA


Phase 2: Use of Radioxenon Monitoring Equipment in Freiburg [1] [2]

The four measurement systems tested in Phase 2 had favorable results in that all of the systems met CTBTO minimum specifications and agreed with the independent analyses provided by BfS.

INGE Phase 3

Phase 3, which was separated into a, b, and c components was designed primarily to test commercial versions of the systems designed and tested in INGE Phase 2. The commercial version of the SAUNA (the SAUNA-II) is now being manufactured by Gammadata, Inc. and the SPALAX Archived 2015-02-13 at the Wayback Machine is being produced commercially by Environnement S.A, Radionuclides Division (formerly Societé Française d’Ingenierie: SFI).

One of the major aspects of the INGE that has been investigated is the variation of worldwide radioactive xenon backgrounds. Concentrations of the xenon isotopes are continuously measured throughout the INGE experiment, and it has been found so far that a major source of background is medical isotope production.

There has been a number of workshops to discuss various aspects of the experiment and to discuss worldwide backgrounds of radioxenon.

1999 - Freiburg, Germany
1999 - Freiburg, Germany
2000 - Freiburg, Germany
2000 - Freiburg, Germany
2001 - Stockholm, Sweden
2002 - Tahiti, French Polynesia
2002 - Richland, Washington, United States
2003 - Ottawa, Canada
2004 - Strassoldo, Italy
2005 - Stockholm, Sweden
2006 - Melbourne, Australia
2007 - Las Vegas, Nevada, United States
2008 - St. Petersburg, Russian Federation
2009 - Daejeon, South Korea
2010 - Buenos Aires, Argentina
2011 - Yogyakarta, Indonesia
2012 - Mito, Japan
2013 - Vienna, Austria
2015 - Austin, Texas, United States
2017 - London, United Kingdom
2019 - Freiburg, Germany

Related Research Articles

<span class="mw-page-title-main">Comprehensive Nuclear-Test-Ban Treaty</span> 1996 treaty banning all nuclear weapons testing

The Comprehensive Nuclear-Test-Ban Treaty (CTBT) is a multilateral treaty to ban nuclear weapons test explosions and any other nuclear explosions, for both civilian and military purposes, in all environments. It was adopted by the United Nations General Assembly on 10 September 1996, but has not entered into force, as eight specific nations have not ratified the treaty.

Radiometric dating, radioactive dating or radioisotope dating is a technique which is used to date materials such as rocks or carbon, in which trace radioactive impurities were selectively incorporated when they were formed. The method compares the abundance of a naturally occurring radioactive isotope within the material to the abundance of its decay products, which form at a known constant rate of decay. The use of radiometric dating was first published in 1907 by Bertram Boltwood and is now the principal source of information about the absolute age of rocks and other geological features, including the age of fossilized life forms or the age of Earth itself, and can also be used to date a wide range of natural and man-made materials.

<span class="mw-page-title-main">Xenon</span> Chemical element with atomic number 54 (Xe)

Xenon is a chemical element; it has symbol Xe and atomic number 54. It is a dense, colorless, odorless noble gas found in Earth's atmosphere in trace amounts. Although generally unreactive, it can undergo a few chemical reactions such as the formation of xenon hexafluoroplatinate, the first noble gas compound to be synthesized.

<span class="mw-page-title-main">Stable nuclide</span> Nuclide that does not undergo radioactive decay

Stable nuclides are nuclides that are not radioactive and so do not spontaneously undergo radioactive decay. When such nuclides are referred to in relation to specific elements, they are usually termed stable isotopes.

<span class="mw-page-title-main">Nuclear medicine</span> Medical specialty

Nuclear medicine, or nucleology, is a medical specialty involving the application of radioactive substances in the diagnosis and treatment of disease. Nuclear imaging is, in a sense, radiology done inside out, because it records radiation emitted from within the body rather than radiation that is transmitted through the body from external sources like X-ray generators. In addition, nuclear medicine scans differ from radiology, as the emphasis is not on imaging anatomy, but on the function. For such reason, it is called a physiological imaging modality. Single photon emission computed tomography (SPECT) and positron emission tomography (PET) scans are the two most common imaging modalities in nuclear medicine.

A radioactive tracer, radiotracer, or radioactive label is a synthetic derivative of a natural compound in which one or more atoms have been replaced by a radionuclide. By virtue of its radioactive decay, it can be used to explore the mechanism of chemical reactions by tracing the path that the radioisotope follows from reactants to products. Radiolabeling or radiotracing is thus the radioactive form of isotopic labeling. In biological contexts, experiments that use radioisotope tracers are sometimes called radioisotope feeding experiments.

<span class="mw-page-title-main">Iodine-131</span> Isotope of iodine

Iodine-131 is an important radioisotope of iodine discovered by Glenn Seaborg and John Livingood in 1938 at the University of California, Berkeley. It has a radioactive decay half-life of about eight days. It is associated with nuclear energy, medical diagnostic and treatment procedures, and natural gas production. It also plays a major role as a radioactive isotope present in nuclear fission products, and was a significant contributor to the health hazards from open-air atomic bomb testing in the 1950s, and from the Chernobyl disaster, as well as being a large fraction of the contamination hazard in the first weeks in the Fukushima nuclear crisis. This is because 131I is a major fission product of uranium and plutonium, comprising nearly 3% of the total products of fission. See fission product yield for a comparison with other radioactive fission products. 131I is also a major fission product of uranium-233, produced from thorium.

Naturally occurring xenon (54Xe) consists of seven stable isotopes and two very long-lived isotopes. Double electron capture has been observed in 124Xe and double beta decay in 136Xe, which are among the longest measured half-lives of all nuclides. The isotopes 126Xe and 134Xe are also predicted to undergo double beta decay, but this process has never been observed in these isotopes, so they are considered to be stable. Beyond these stable forms, 32 artificial unstable isotopes and various isomers have been studied, the longest-lived of which is 127Xe with a half-life of 36.345 days. All other isotopes have half-lives less than 12 days, most less than 20 hours. The shortest-lived isotope, 108Xe, has a half-life of 58 μs, and is the heaviest known nuclide with equal numbers of protons and neutrons. Of known isomers, the longest-lived is 131mXe with a half-life of 11.934 days. 129Xe is produced by beta decay of 129I ; 131mXe, 133Xe, 133mXe, and 135Xe are some of the fission products of both 235U and 239Pu, so are used as indicators of nuclear explosions.

<span class="mw-page-title-main">Isotopes of iodine</span> Nuclides with atomic number of 53 but with different mass numbers

There are 40 known isotopes of iodine (53I) from 108I to 147I; all undergo radioactive decay except 127I, which is stable. Iodine is thus a monoisotopic element.

Caesium (55Cs) has 41 known isotopes, the atomic masses of these isotopes range from 112 to 152. Only one isotope, 133Cs, is stable. The longest-lived radioisotopes are 135Cs with a half-life of 1.33 million years, 137
Cs
with a half-life of 30.1671 years and 134Cs with a half-life of 2.0652 years. All other isotopes have half-lives less than 2 weeks, most under an hour.

The Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) is an international organization that will be established upon the entry into force of the Comprehensive Nuclear-Test-Ban Treaty, a Convention that outlaws nuclear test explosions. Its seat will be in Vienna, Austria. The organization will be tasked with verifying the ban on nuclear tests and will operate therefore a worldwide monitoring system and may conduct on-site inspections. The Preparatory Commission for the CTBTO, and its Provisional Technical Secretariat, were established in 1997 and are headquartered in Vienna, Austria.

Iodine-125 (125I) is a radioisotope of iodine which has uses in biological assays, nuclear medicine imaging and in radiation therapy as brachytherapy to treat a number of conditions, including prostate cancer, uveal melanomas, and brain tumors. It is the second longest-lived radioisotope of iodine, after iodine-129.

Iodine-123 (123I) is a radioactive isotope of iodine used in nuclear medicine imaging, including single-photon emission computed tomography (SPECT) or SPECT/CT exams. The isotope's half-life is 13.2232 hours; the decay by electron capture to tellurium-123 emits gamma radiation with a predominant energy of 159 keV. In medical applications, the radiation is detected by a gamma camera. The isotope is typically applied as iodide-123, the anionic form.

A radio-frequency quadrupole (RFQ) beam cooler is a device for particle beam cooling, especially suited for ion beams. It lowers the temperature of a particle beam by reducing its energy dispersion and emittance, effectively increasing its brightness (brilliance). The prevalent mechanism for cooling in this case is buffer-gas cooling, whereby the beam loses energy from collisions with a light, neutral and inert gas. The cooling must take place within a confining field in order to counteract the thermal diffusion that results from the ion-atom collisions.

Iodine-129 (129I) is a long-lived radioisotope of iodine that occurs naturally but is also of special interest in the monitoring and effects of man-made nuclear fission products, where it serves as both a tracer and a potential radiological contaminant.

<span class="mw-page-title-main">Automated radioxenon sampler analyzer</span>

The automated radioxenon sampler-analyzer (ARSA) was designed by the Pacific Northwest National Laboratory in the late 1990s with funding and support from the U.S. Department of Energy. The ARSA system automatically collects and measures radioxenon from the air.

An extinct radionuclide is a radionuclide that was formed by nucleosynthesis before the formation of the Solar System, about 4.6 billion years ago, but has since decayed to virtually zero abundance and is no longer detectable as a primordial nuclide. Extinct radionuclides were generated by various processes in the early Solar system, and became part of the composition of meteorites and protoplanets. All widely documented extinct radionuclides have half-lives shorter than 100 million years.

<span class="mw-page-title-main">Primordial nuclide</span> Nuclides predating the Earths formation (found on Earth)

In geochemistry, geophysics and nuclear physics, primordial nuclides, also known as primordial isotopes, are nuclides found on Earth that have existed in their current form since before Earth was formed. Primordial nuclides were present in the interstellar medium from which the solar system was formed, and were formed in, or after, the Big Bang, by nucleosynthesis in stars and supernovae followed by mass ejection, by cosmic ray spallation, and potentially from other processes. They are the stable nuclides plus the long-lived fraction of radionuclides surviving in the primordial solar nebula through planet accretion until the present; 286 such nuclides are known.

<span class="mw-page-title-main">Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization</span> Intergovernmental organization for nuclear-test banning

The Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization, or CTBTO Preparatory Commission, is an international organization based in Vienna, Austria, that is tasked with building up the verification regime of the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO). The organization was established by the States Signatories to the Comprehensive Nuclear-Test-Ban Treaty (CTBT) in 1996.

A nuclear detonation detection system (NDDS) is a device or a series of devices that are able to indicate, and pinpoint a nuclear explosion has occurred as well as the direction of the explosion. The main purpose of these devices or systems was to verify compliance of countries that signed nuclear treaties such as the Partial Test Ban treaty of 1963 (PTBT) and the Treaty of Tlatelolco.

References

  1. Auer M., A. Axelsson, X. Blanchard, T.W. Bowyer, G. Brachet, I. Bulowski, Y. Dubasov, K. Elmgren, J.P. Fontaine, W. Harms, J.C. Hayes, T.R. Heimbigner, J.I. McIntyre, M.E. Panisko, Y. Popov, A. Ringbom, H. Sartorius, S. Schmid, J. Schulze, C. Schlosser, T. Taffary, W. Weiss, and B. Wernsperger. 2004. Intercomparison experiments of systems for the measurement of xenon radionuclides in the atmosphere. Applied Radiation and Isotopes 60:863–877.
  2. Bowyer, T.W., C. Schlosser, K.H. Abel, M. Auer, J.C. Hayes, T.R. Heimbigner, J.I. McIntyre, M.E. Panisko, P.L. Reeder, H. Sartorius, J. Schulze, and W. Weiss. 2002. Detection and analysis of xenon isotopes for the Comprehensive Nuclear-Test-Ban Treaty international monitoring system. Journal of Environmental Radioactivity 59:139–151.