Quantum oscillations (experimental technique)

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Condensed matter
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Neutron scattering
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In condensed matter physics, Quantum oscillations describes a series of related experimental techniques used to map the Fermi surface of a metal in the presence of a strong magnetic field. [1] These techniques are based on the principle of Landau quantization of Fermions moving in a magnetic field. [2] For a gas of free fermions in a strong magnetic field, the energy levels are quantized into bands, called the Landau levels, whose separation is proportional to the strength of the magnetic field. In a quantum oscillation experiment, the external magnetic field is varied, which causes the Landau levels to pass over the Fermi surface, which in turn results in oscillations of the electronic density of states at the Fermi level; this produces oscillations in the many material properties which depend on this, including resistance (the Shubnikov-de Haas effect), Hall resistance, [2] and magnetic susceptibility (the de Haas-van Alphen effect). Observation of quantum oscillations in a material is considered a signature of Fermi liquid behaviour. [3]

Contents

Quantum oscillations have been used to study high temperature superconducting materials such as cuprates and pnictides. [1] Studies using these experiments have shown that the ground state of underdoped cuprates behave similar to a Fermi liquid, and display characteristics such as Landau quasiparticles. [4]

In 2021 this technique has been used to observe a predicted state called "electron-phonon fluid", [5] [6] a similar particle-quasiparticle state already known is the exciton-polariton fluid

Experiment

When a magnetic field is applied to a system of free charged fermions, their energy states are quantized into the so-called Landau levels, given by [7]

YBCO superconductor under high magnetic field. As field strength is increased, superconductivity is suppressed and Landau oscillations can be observed Quantum oscillations at 100 T.jpg
YBCO superconductor under high magnetic field. As field strength is increased, superconductivity is suppressed and Landau oscillations can be observed

for integer-valued , where is the external magnetic field and are the fermion charge and effective mass respectively.

When the external magnetic field is increased in an isolated system, the Landau levels expand, and eventually "fall off" the Fermi surface. This leads to oscillations in the observed energy of the highest occupied level, and hence in many physical properties (including Hall conductivity, resistivity, and susceptibility). The periodicity of these oscillations can be measured, and in turn can be used to determine the cross-sectional area of the Fermi surface. [8] If the axis of the magnetic field is varied at constant magnitude, similar oscillations are observed. The oscillations occur whenever the Landau orbits touch the Fermi surface. In this way, the complete geometry of the Fermi sphere can be mapped. [8]

Underdoped cuprates

Studies of underdoped cuprate compounds such as YBa2Cu3O6+x through probes such as ARPES have indicated that these phases show characteristics of non-Fermi liquids, [9] and in particular, the absence of well-defined Landau quasiparticles. [10] However, quantum oscillations have been observed in these materials at low temperatures, if their superconductivity is suppressed by a sufficiently high magnetic field, [2] which is evidence for the presence of well-defined quasiparticles with fermionic statistics. These experimental results thus disagree with those from ARPES and other probes. [7]

See also

Related Research Articles

Condensed matter physics Branch of physics dealing with a property of matter

Condensed matter physics is the field of physics that deals with the macroscopic and microscopic physical properties of matter, especially the solid and liquid phases which arise from electromagnetic forces between atoms. More generally, the subject deals with "condensed" phases of matter: systems of many constituents with strong interactions between them. More exotic condensed phases include the superconducting phase exhibited by certain materials at low temperature, the ferromagnetic and antiferromagnetic phases of spins on crystal lattices of atoms, and the Bose–Einstein condensate found in ultracold atomic systems. Condensed matter physicists seek to understand the behavior of these phases by experiments to measure various material properties, and by applying the physical laws of quantum mechanics, electromagnetism, statistical mechanics, and other theories to develop mathematical models.

The quantum Hall effect is a quantized version of the Hall effect which is observed in two-dimensional electron systems subjected to low temperatures and strong magnetic fields, in which the Hall resistance Rxy exhibits steps that take on the quantized values

Fermi liquid theory

Fermi liquid theory is a theoretical model of interacting fermions that describes the normal state of most metals at sufficiently low temperatures. The interactions among the particles of the many-body system do not need to be small. The phenomenological theory of Fermi liquids was introduced by the Soviet physicist Lev Davidovich Landau in 1956, and later developed by Alexei Abrikosov and Isaak Khalatnikov using diagrammatic perturbation theory. The theory explains why some of the properties of an interacting fermion system are very similar to those of the ideal Fermi gas, and why other properties differ.

In physics, an anyon is a type of quasiparticle that occurs only in two-dimensional systems, with properties much less restricted than the two kinds of standard elementary particles, fermions and bosons. In general, the operation of exchanging two identical particles, although it may cause a global phase shift, cannot affect observables. Anyons are generally classified as abelian or non-abelian. Abelian anyons play a major role in the fractional quantum Hall effect. Non-abelian anyons have not been definitively detected, although this is an active area of research.

In physics, quasiparticles and collective excitations are emergent phenomena that occur when a microscopically complicated system such as a solid behaves as if it contained different weakly interacting particles in vacuum. For example, as an electron travels through a semiconductor, its motion is disturbed in a complex way by its interactions with other electrons and with atomic nuclei. The electron behaves as though it has a different effective mass travelling unperturbed in vacuum. Such an electron is called an electron quasiparticle. In another example, the aggregate motion of electrons in the valence band of a semiconductor or a hole band in a metal behave as though the material instead contained positively charged quasiparticles called electron holes. Other quasiparticles or collective excitations include the phonon, the plasmons, and many others.

Luttinger liquid Theoretical model describing interacting fermions in a one-dimensional conductor

A Luttinger liquid, or Tomonaga–Luttinger liquid, is a theoretical model describing interacting electrons in a one-dimensional conductor. Such a model is necessary as the commonly used Fermi liquid model breaks down for one dimension.

In condensed matter physics, the Fermi surface is the surface in reciprocal space which separates occupied from unoccupied electron states at zero temperature. The shape of the Fermi surface is derived from the periodicity and symmetry of the crystalline lattice and from the occupation of electronic energy bands. The existence of a Fermi surface is a direct consequence of the Pauli exclusion principle, which allows a maximum of one electron per quantum state. The study of the Fermi surfaces of materials is called fermiology.

The fractional quantum Hall effect (FQHE) is a physical phenomenon in which the Hall conductance of 2D electrons shows precisely quantised plateaus at fractional values of . It is a property of a collective state in which electrons bind magnetic flux lines to make new quasiparticles, and excitations have a fractional elementary charge and possibly also fractional statistics. The 1998 Nobel Prize in Physics was awarded to Robert Laughlin, Horst Störmer, and Daniel Tsui "for their discovery of a new form of quantum fluid with fractionally charged excitations" Laughlin's explanation only applies to fillings where is an odd integer. The microscopic origin of the FQHE is a major research topic in condensed matter physics.

Pseudogap State at which a Fermi surface has a partial energy gap in condensed matter physics

In condensed matter physics, a pseudogap describes a state where the Fermi surface of a material possesses a partial energy gap, for example, a band structure state where the Fermi surface is gapped only at certain points. The term pseudogap was coined by Nevill Mott in 1968 to indicate a minimum in the density of states at the Fermi level, N(EF), resulting from Coulomb repulsion between electrons in the same atom, a band gap in a disordered material or a combination of these. In the modern context pseudogap is a term from the field of high-temperature superconductivity which refers to an energy range which has very few states associated with it. This is very similar to a true 'gap', which is an energy range that contains no allowed states. Such gaps open up, for example, when electrons interact with the lattice. The pseudogap phenomenon is observed in a region of the phase diagram generic to cuprate high-temperature superconductors, existing in underdoped specimens at temperatures above the superconducting transition temperature.

Type-II superconductor Superconductor characterized by the formation of magnetic vortices in an applied magnetic field

In superconductivity, a type-II superconductor is a superconductor that exhibits an intermediate phase of mixed ordinary and superconducting properties at intermediate temperature and fields above the superconducting phases. It also features the formation of magnetic field vortices with an applied external magnetic field. This occurs above a certain critical field strength Hc1. The vortex density increases with increasing field strength. At a higher critical field Hc2, superconductivity is destroyed. Type-II superconductors do not exhibit a complete Meissner effect.

Majorana fermion Fermion that is its own antiparticle

A Majorana fermion, also referred to as a Majorana particle, is a fermion that is its own antiparticle. They were hypothesised by Ettore Majorana in 1937. The term is sometimes used in opposition to a Dirac fermion, which describes fermions that are not their own antiparticles.

The De Haas–Van Alphen effect, often abbreviated to DHVA, is a quantum mechanical effect in which the magnetic susceptibility of a pure metal crystal oscillates as the intensity of the magnetic field B is increased. It can be used to determine the Fermi surface of a material. Other quantities also oscillate, such as the electrical resistivity, specific heat, and sound attenuation and speed. It is named after Wander Johannes de Haas and his student Pieter M. van Alphen. The DHVA effect comes from the orbital motion of itinerant electrons in the material. An equivalent phenomenon at low magnetic fields is known as Landau diamagnetism.

An oscillation in the conductivity of a material that occurs at low temperatures in the presence of very intense magnetic fields, the Shubnikov–de Haas effect (SdH) is a macroscopic manifestation of the inherent quantum mechanical nature of matter. It is often used to determine the effective mass of charge carriers, allowing investigators to distinguish among majority and minority carrier populations. The effect is named after Wander Johannes de Haas and Lev Shubnikov.

In solid-state physics, heavy fermion materials are a specific type of intermetallic compound, containing elements with 4f or 5f electrons in unfilled electron bands. Electrons are one type of fermion, and when they are found in such materials, they are sometimes referred to as heavy electrons. Heavy fermion materials have a low-temperature specific heat whose linear term is up to 1000 times larger than the value expected from the free electron model. The properties of the heavy fermion compounds often derive from the partly filled f-orbitals of rare-earth or actinide ions, which behave like localized magnetic moments. The name "heavy fermion" comes from the fact that the fermion behaves as if it has an effective mass greater than its rest mass. In the case of electrons, below a characteristic temperature (typically 10 K), the conduction electrons in these metallic compounds behave as if they had an effective mass up to 1000 times the free particle mass. This large effective mass is also reflected in a large contribution to the resistivity from electron-electron scattering via the Kadowaki–Woods ratio. Heavy fermion behavior has been found in a broad variety of states including metallic, superconducting, insulating and magnetic states. Characteristic examples are CeCu6, CeAl3, CeCu2Si2, YbAl3, UBe13 and UPt3.

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References

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