Magneto-optic effect

Last updated

A magneto-optic effect is any one of a number of phenomena in which an electromagnetic wave propagates through a medium that has been altered by the presence of a quasistatic magnetic field. In such a medium, which is also called gyrotropic or gyromagnetic, left- and right-rotating elliptical polarizations can propagate at different speeds, leading to a number of important phenomena. When light is transmitted through a layer of magneto-optic material, the result is called the Faraday effect: the plane of polarization can be rotated, forming a Faraday rotator. The results of reflection from a magneto-optic material are known as the magneto-optic Kerr effect (not to be confused with the nonlinear Kerr effect).

Contents

In general, magneto-optic effects break time reversal symmetry locally (i.e. when only the propagation of light, and not the source of the magnetic field, is considered) as well as Lorentz reciprocity, which is a necessary condition to construct devices such as optical isolators (through which light passes in one direction but not the other).

Two gyrotropic materials with reversed rotation directions of the two principal polarizations, corresponding to complex-conjugate ε tensors for lossless media, are called optical isomers.

Gyrotropic permittivity

In particular, in a magneto-optic material the presence of a magnetic field (either externally applied or because the material itself is ferromagnetic) can cause a change in the permittivity tensor ε of the material. The ε becomes anisotropic, a 3×3 matrix, with complex off-diagonal components, depending on the frequency ω of incident light. If the absorption losses can be neglected, ε is a Hermitian matrix. The resulting principal axes become complex as well, corresponding to elliptically-polarized light where left- and right-rotating polarizations can travel at different speeds (analogous to birefringence).

More specifically, for the case where absorption losses can be neglected, the most general form of Hermitian ε is:

or equivalently the relationship between the displacement field D and the electric field E is:

where is a real symmetric matrix and is a real pseudovector called the gyration vector, whose magnitude is generally small compared to the eigenvalues of . The direction of g is called the axis of gyration of the material. To first order, g is proportional to the applied magnetic field:

where is the magneto-optical susceptibility (a scalar in isotropic media, but more generally a tensor). If this susceptibility itself depends upon the electric field, one can obtain a nonlinear optical effect of magneto-optical parametric generation (somewhat analogous to a Pockels effect whose strength is controlled by the applied magnetic field).

The simplest case to analyze is the one in which g is a principal axis (eigenvector) of , and the other two eigenvalues of are identical. Then, if we let g lie in the z direction for simplicity, the ε tensor simplifies to the form:

Most commonly, one considers light propagating in the z direction (parallel to g). In this case the solutions are elliptically polarized electromagnetic waves with phase velocities (where μ is the magnetic permeability). This difference in phase velocities leads to the Faraday effect.

For light propagating purely perpendicular to the axis of gyration, the properties are known as the Cotton-Mouton effect and used for a Circulator.

Kerr rotation and Kerr ellipticity

Kerr rotation and Kerr ellipticity are changes in the polarization of incident light which comes in contact with a gyromagnetic material. Kerr rotation is a rotation in the plane of polarization of transmitted light, and Kerr ellipticity is the ratio of the major to minor axis of the ellipse traced out by elliptically polarized light on the plane through which it propagates. Changes in the orientation of polarized incident light can be quantified using these two properties.

Circular Polarized Light Circular.Polarization.Circularly.Polarized.Light With.Components Right.Handed.svg
Circular Polarized Light

According to classical physics, the speed of light varies with the permittivity of a material:

where is the velocity of light through the material, is the material permittivity, and is the material permeability. Because the permittivity is anisotropic, polarized light of different orientations will travel at different speeds.

This can be better understood if we consider a wave of light that is circularly polarized (seen to the right). If this wave interacts with a material at which the horizontal component (green sinusoid) travels at a different speed than the vertical component (blue sinusoid), the two components will fall out of the 90 degree phase difference (required for circular polarization) changing the Kerr ellipticity.

A change in Kerr rotation is most easily recognized in linearly polarized light, which can be separated into two circularly polarized components: Left-handed circular polarized (LHCP) light and right-handed circular polarized (RHCP) light. The anisotropy of the magneto-optic material permittivity causes a difference in the speed of LHCP and RHCP light, which will cause a change in the angle of polarized light. Materials that exhibit this property are known as birefringent.

From this rotation, we can calculate the difference in orthogonal velocity components, find the anisotropic permittivity, find the gyration vector, and calculate the applied magnetic field [1] .

See also

Related Research Articles

In optics, polarized light can be described using the Jones calculus, discovered by R. C. Jones in 1941. Polarized light is represented by a Jones vector, and linear optical elements are represented by Jones matrices. When light crosses an optical element the resulting polarization of the emerging light is found by taking the product of the Jones matrix of the optical element and the Jones vector of the incident light. Note that Jones calculus is only applicable to light that is already fully polarized. Light which is randomly polarized, partially polarized, or incoherent must be treated using Mueller calculus.

<span class="mw-page-title-main">Refractive index</span> Ratio of the speed of light in vacuum to that in the medium

In optics, the refractive index of an optical medium is a dimensionless number that gives the indication of the light bending ability of that medium.

<span class="mw-page-title-main">Optical rotation</span> Concept in enantioselective synthesis

Optical rotation, also known as polarization rotation or circular birefringence, is the rotation of the orientation of the plane of polarization about the optical axis of linearly polarized light as it travels through certain materials. Circular birefringence and circular dichroism are the manifestations of optical activity. Optical activity occurs only in chiral materials, those lacking microscopic mirror symmetry. Unlike other sources of birefringence which alter a beam's state of polarization, optical activity can be observed in fluids. This can include gases or solutions of chiral molecules such as sugars, molecules with helical secondary structure such as some proteins, and also chiral liquid crystals. It can also be observed in chiral solids such as certain crystals with a rotation between adjacent crystal planes or metamaterials.

<span class="mw-page-title-main">Circular polarization</span> Polarization state

In electrodynamics, circular polarization of an electromagnetic wave is a polarization state in which, at each point, the electromagnetic field of the wave has a constant magnitude and is rotating at a constant rate in a plane perpendicular to the direction of the wave.

In electrodynamics, elliptical polarization is the polarization of electromagnetic radiation such that the tip of the electric field vector describes an ellipse in any fixed plane intersecting, and normal to, the direction of propagation. An elliptically polarized wave may be resolved into two linearly polarized waves in phase quadrature, with their polarization planes at right angles to each other. Since the electric field can rotate clockwise or counterclockwise as it propagates, elliptically polarized waves exhibit chirality.

In electrodynamics, linear polarization or plane polarization of electromagnetic radiation is a confinement of the electric field vector or magnetic field vector to a given plane along the direction of propagation. The term linear polarization was coined by Augustin-Jean Fresnel in 1822. See polarization and plane of polarization for more information.

<span class="mw-page-title-main">Polarization (physics)</span> Property of waves that can oscillate with more than one orientation

Polarization is a property of transverse waves which specifies the geometrical orientation of the oscillations. In a transverse wave, the direction of the oscillation is perpendicular to the direction of motion of the wave. A simple example of a polarized transverse wave is vibrations traveling along a taut string (see image); for example, in a musical instrument like a guitar string. Depending on how the string is plucked, the vibrations can be in a vertical direction, horizontal direction, or at any angle perpendicular to the string. In contrast, in longitudinal waves, such as sound waves in a liquid or gas, the displacement of the particles in the oscillation is always in the direction of propagation, so these waves do not exhibit polarization. Transverse waves that exhibit polarization include electromagnetic waves such as light and radio waves, gravitational waves, and transverse sound waves in solids.

<span class="mw-page-title-main">Waveplate</span> Optical polarization device

A waveplate or retarder is an optical device that alters the polarization state of a light wave travelling through it. Two common types of waveplates are the half-wave plate, which shifts the polarization direction of linearly polarized light, and the quarter-wave plate, which converts linearly polarized light into circularly polarized light and vice versa. A quarter-wave plate can be used to produce elliptical polarization as well.

<span class="mw-page-title-main">Permittivity</span> Measure of the electric polarizability of a dielectric

In electromagnetism, the absolute permittivity, often simply called permittivity and denoted by the Greek letter ε (epsilon), is a measure of the electric polarizability of a dielectric. A material with high permittivity polarizes more in response to an applied electric field than a material with low permittivity, thereby storing more energy in the material. In electrostatics, the permittivity plays an important role in determining the capacitance of a capacitor.

Circular dichroism (CD) is dichroism involving circularly polarized light, i.e., the differential absorption of left- and right-handed light. Left-hand circular (LHC) and right-hand circular (RHC) polarized light represent two possible spin angular momentum states for a photon, and so circular dichroism is also referred to as dichroism for spin angular momentum. This phenomenon was discovered by Jean-Baptiste Biot, Augustin Fresnel, and Aimé Cotton in the first half of the 19th century. Circular dichroism and circular birefringence are manifestations of optical activity. It is exhibited in the absorption bands of optically active chiral molecules. CD spectroscopy has a wide range of applications in many different fields. Most notably, UV CD is used to investigate the secondary structure of proteins. UV/Vis CD is used to investigate charge-transfer transitions. Near-infrared CD is used to investigate geometric and electronic structure by probing metal d→d transitions. Vibrational circular dichroism, which uses light from the infrared energy region, is used for structural studies of small organic molecules, and most recently proteins and DNA.

Crystal optics is the branch of optics that describes the behaviour of light in anisotropic media, that is, media in which light behaves differently depending on which direction the light is propagating. The index of refraction depends on both composition and crystal structure and can be calculated using the Gladstone–Dale relation. Crystals are often naturally anisotropic, and in some media it is possible to induce anisotropy by applying an external electric field.

<span class="mw-page-title-main">Birefringence</span> Optical phenomenon

Birefringence is the optical property of a material having a refractive index that depends on the polarization and propagation direction of light. These optically anisotropic materials are said to be birefringent. The birefringence is often quantified as the maximum difference between refractive indices exhibited by the material. Crystals with non-cubic crystal structures are often birefringent, as are plastics under mechanical stress.

The Faraday effect or Faraday rotation, sometimes referred to as the magneto-optic Faraday effect (MOFE), is a physical magneto-optical phenomenon. The Faraday effect causes a polarization rotation which is proportional to the projection of the magnetic field along the direction of the light propagation. Formally, it is a special case of gyroelectromagnetism obtained when the dielectric permittivity tensor is diagonal. This effect occurs in most optically transparent dielectric materials under the influence of magnetic fields.

<span class="mw-page-title-main">Faraday rotator</span>

A Faraday rotator is a polarization rotator based on the Faraday effect, a magneto-optic effect involving transmission of light through a material when a longitudinal static magnetic field is present. The state of polarization is rotated as the wave traverses the device, which is explained by a slight difference in the phase velocity between the left and right circular polarizations. Thus it is an example of circular birefringence, as is optical activity, but involves a material only having this property in the presence of a magnetic field. Circular birefringence, involving a difference in propagation between opposite circular polarizations, is distinct from linear birefringence which also transforms a wave's polarization but not through a simple rotation.

The Kerr effect, also called the quadratic electro-optic (QEO) effect, is a change in the refractive index of a material in response to an applied electric field. The Kerr effect is distinct from the Pockels effect in that the induced index change is directly proportional to the square of the electric field instead of varying linearly with it. All materials show a Kerr effect, but certain liquids display it more strongly than others. The Kerr effect was discovered in 1875 by Scottish physicist John Kerr.

Polarizability usually refers to the tendency of matter, when subjected to an electric field, to acquire an electric dipole moment in proportion to that applied field. It is a property of all matter, considering that matter is made up of elementary particles which have an electric charge, namely protons and electrons. When subject to an electric field, the negatively charged electrons and positively charged atomic nuclei are subject to opposite forces and undergo charge separation. Polarizability is responsible for a material's dielectric constant and, at high (optical) frequencies, its refractive index.

<span class="mw-page-title-main">Magneto-optic Kerr effect</span>

In physics the magneto-optic Kerr effect (MOKE) or the surface magneto-optic Kerr effect (SMOKE) is one of the magneto-optic effects. It describes the changes to light reflected from a magnetized surface. It is used in materials science research in devices such as the Kerr microscope, to investigate the magnetization structure of materials.

<span class="mw-page-title-main">Voigt effect</span>

The Voigt effect is a magneto-optical phenomenon which rotates and elliptizes linearly polarised light sent into an optically active medium. Unlike many other magneto-optical effects such as the Kerr or Faraday effect which are linearly proportional to the magnetization, the Voigt effect is proportional to the square of the magnetization and can be seen experimentally at normal incidence. There are several denominations for this effect in the literature: the Cotton–Mouton effect, the Voigt effect, and magnetic-linear birefringence. This last denomination is closer in the physical sense, where the Voigt effect is a magnetic birefringence of the material with an index of refraction parallel and perpendicular ) to the magnetization vector or to the applied magnetic field.

<span class="mw-page-title-main">Angular momentum of light</span> Physical quantity carried in photons

The angular momentum of light is a vector quantity that expresses the amount of dynamical rotation present in the electromagnetic field of the light. While traveling approximately in a straight line, a beam of light can also be rotating around its own axis. This rotation, while not visible to the naked eye, can be revealed by the interaction of the light beam with matter.

The spin angular momentum of light (SAM) is the component of angular momentum of light that is associated with the quantum spin and the rotation between the polarization degrees of freedom of the photon.

References

  1. Garcia-Merino, J. A. "Magneto-conductivity and magnetically-controlled nonlinear optical transmittance in multi-wall carbon nanotubes". Optics Express. 24 (17): 19552–19557. doi: 10.1364/OE.24.019552 .

PD-icon.svg This article incorporates public domain material from Federal Standard 1037C. General Services Administration. Archived from the original on 2022-01-22.