MIRACLS experiment

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Isotope Separator On Line Device
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COLLAPS, CRIS, EC-SLI, IDS, ISS, ISOLTRAP, LUCRECIA, Miniball, MIRACLS, SEC, VITO, WISArD
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MR-ToF Mirrors of the MIRACLS Experiment MIRACLS MR-ToF.jpg
MR-ToF Mirrors of the MIRACLS Experiment

The Multi Ion Reflection Apparatus for Colinear Laser Spectroscopy (MIRACLS) is a permanent experiment setup being constructed at the ISOLDE facility at CERN. The purpose of the experiment is to measure properties of exotic radioisotopes, from precise measurements of their hyperfine structure. MIRACLS will use laser spectroscopy for measurements, aiming to increase the sensitivity of the technique by trapping ion bunches in an ion trap. [1]

Contents

Background

Collinear laser spectroscopy is a technique allowing the measurements of properties of nuclei, such as ground state spins, electromagnetic moments and charge radii. The technique uses a narrow radioactive ion beam (RIB) of a specific isotope and overlaps it with a narrow-band, continuous-wave laser beam of specific frequency. The laser is tuned to match the energy difference between the atomic energy levels of interest, which leads to a resonant absorption or emission of photons by the atoms. [2]

Multi-reflection time-of-flight (MR-ToF) instruments reflect an ion bunch between two electrostatic mirrors, so that the flight path of the ion is increased to the orders of kilometres. The device mass separates the ions in addition to increasing their flight path, as different masses will have different times of flight. [3]

Paul trap for the MIRACLS experiment MIRACLS Paul Trap.jpg
Paul trap for the MIRACLS experiment

A Paul trap, also referred to as a quadrupole ion trap or a radio frequency (RF) trap, is an ion trap that uses dynamic electric fields to trap charged particles. It is not possible to create a configuration of static electricity fields to trap the particles in three dimensions, however it is possible with dynamic electric fields. The confining and anti-confining directions are switched at a rate faster that it takes the particle to escape the trap.

Experimental setup

The MIRACLS proof-of-principle setup consists of an electron-impact ion source providing a continuous, stable magnesium ion beam. [4] The beam is injected into a helium-buffer gas-filled Paul trap which cools and accumulates it into defined ion bunches. [5] The bunches pass an electrostatic quadrupole bender and enter the MR-ToF region where they are decelerated and captured. [4]

The MR-ToF consists of two electrostatic mirrors, which are made of four cylindrical electrodes with electric potential applied. [4] The potentials are set to optimise trapping and focusing, whilst also keeping the central drift region of the device free of fringe (outer magnetic) fields. [6] This region is surrounded by a mesh electrode that controls the electric potential and provides an enhanced photon transparency near the optical detection region (ODR). [7] The ODR consists of an optical lens system and photomultiplier tube (PMT) to detect fluorescence photons emitted by the excited Mg+ ions, mounted above the mesh electrode. [8] The system is surrounded by a stray light shield to block out photons not originating from the ions in the ODR. [9]

The narrow-band, continuous-wave laser beam enters the setup through a quartz window, at the first electrostatic quadrupole bender. [10] It is overlapped with the axis of the MR-ToF device, and at resonance with the (Doppler-shifted) optical transition photons are detected in the PMT. [4]

The ion bunches are ejected from the MR-ToF by the in-trap lift mechanism and pass a second electron quadrupole bender. [4] They are then recorded on a multi-channel place detector (MCP) so that they can be monitored. [6]

MIRACLS aims to increase the sensitivity of the fluorescence collinear laser spectroscopy technique, conventionally used for hyperfine measurements (e.g. COLLAPS). It is improved as during every revolution in the MR-ToF the ion bunches pass the ODR and therefore a higher count of photons is recorded. [4]

Results

Currently, the MIRACLS experiment is being designed and constructed, and therefore only simulated and proof-of-concept results exist. Both sets of results demonstrate the potential of MIRACLS, with the prediction that the first measurements will be performed on neutron-rich Mg and Cadmium isotopes. [6]

Related Research Articles

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<span class="mw-page-title-main">Laser cooling</span> Class of methods for cooling atoms to very low temperatures

Laser cooling includes a number of techniques where atoms, molecules, and small mechanical systems are cooled with laser light. The directed energy of lasers is often associated with heating materials, e.g. laser cutting, so it can be counterintuitive that laser cooling often results in sample temperatures approaching absolute zero. Laser cooling relies on the change in momentum when an object, such as an atom, absorbs and re-emits a photon. For example, if laser light illuminates a warm cloud of atoms from all directions and the laser's frequency is tuned below an atomic resonance, the atoms will be cooled. This common type of laser cooling relies on the Doppler effect where individual atoms will preferentially absorb laser light from the direction opposite to the atom's motion. The absorbed light is re-emitted by the atom in a random direction. After repeated emission and absorption of light the net effect on the cloud of atoms is that they will expand more slowly. The slower expansion reflects a decrease in the velocity distribution of the atoms, which corresponds to a lower temperature and therefore the atoms have been cooled. For an ensemble of particles, their thermodynamic temperature is proportional to the variance in their velocity. More homogeneous velocities between particles corresponds to a lower temperature. Laser cooling techniques combine atomic spectroscopy with the aforementioned mechanical effect of light to compress the velocity distribution of an ensemble of particles, thereby cooling the particles.

<span class="mw-page-title-main">Mass spectrometry</span> Analytical technique based on determining mass to charge ratio of ions

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In atomic physics, hyperfine structure is defined by small shifts in otherwise degenerate energy levels and the resulting splittings in those energy levels of atoms, molecules, and ions, due to electromagnetic multipole interaction between the nucleus and electron clouds.

A microprobe is an instrument that applies a stable and well-focused beam of charged particles to a sample.

<span class="mw-page-title-main">ISOLDE</span> Physics facility at CERN

The ISOLDE Radioactive Ion Beam Facility, is an on-line isotope separator facility located at the centre of the CERN accelerator complex on the Franco-Swiss border. Created in 1964, the ISOLDE facility started delivering radioactive ion beams (RIBs) to users in 1967. Originally located at the Synchro-Cyclotron (SC) accelerator, the facility has been upgraded several times most notably in 1992 when the whole facility was moved to be connected to CERN's ProtonSynchroton Booster (PSB). ISOLDE is currently the longest-running facility in operation at CERN, with continuous developments of the facility and its experiments keeping ISOLDE at the forefront of science with RIBs. ISOLDE benefits a wide range of physics communities with applications covering nuclear, atomic, molecular and solid-state physics, but also biophysics and astrophysics, as well as high-precision experiments looking for physics beyond the Standard Model. The facility is operated by the ISOLDE Collaboration, comprising CERN and sixteen (mostly) European countries. As of 2019, close to 1,000 experimentalists around the world are coming to ISOLDE to perform typically 50 different experiments per year.

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<span class="mw-page-title-main">Electron beam ion trap</span>

Electron beam ion trap (EBIT) is an electromagnetic bottle that produces and confines highly charged ions. An EBIT uses an electron beam focused with a powerful magnetic field to ionize atoms to high charge states by successive electron impact.

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Saturated absorption spectroscopy measures the transition frequency of an atom or molecule between its ground state and an excited state. In saturated absorption spectroscopy, two counter-propagating, overlapped laser beams are sent through a sample of atomic gas. One of the beams stimulates photon emission in excited atoms or molecules when the laser's frequency matches the transition frequency. By changing the laser frequency until these extra photons appear, one can find the exact transition frequency. This method enables precise measurements at room temperature because it is insensitive to doppler broadening. Absorption spectroscopy measures the doppler-broadened transition, so the atoms must be cooled to millikelvin temperatures to achieve the same sensitivity as saturated absorption spectroscopy.

In atomic physics, Raman cooling is a sub-recoil cooling technique that allows the cooling of atoms using optical methods below the limitations of Doppler cooling, Doppler cooling being limited by the recoil energy of a photon given to an atom. This scheme can be performed in simple optical molasses or in molasses where an optical lattice has been superimposed, which are called respectively free space Raman cooling and Raman sideband cooling. Both techniques make use of Raman scattering of laser light by the atoms.

<span class="mw-page-title-main">Peter E. Toschek</span> German physicist (1933–2020)

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<span class="mw-page-title-main">COLLAPS experiment</span>

The COLinear LAser SPectroscopy (COLLAPS) experiment is located in the ISOLDE facility at CERN. The purpose of the experiment is to investigate ground and isomeric state properties of exotic, short lived nuclei, including spins, electro-magnetic moments and charge radii. The experiment has been operating since the late 1970s, and is the oldest active experiment at ISOLDE.

<span class="mw-page-title-main">CRIS experiment</span>

The Collinear Resonance Ionization Spectroscopy (CRIS) experiment is located in the ISOLDE facility at CERN. The experiment aims to study ground-state properties of exotic nuclei and produce high purity isomeric beams used for decay studies. CRIS does this by using the high resolution technique of fast beam collinear laser spectroscopy, with the high efficiency technique of resonance ionization.

<span class="mw-page-title-main">ISOLTRAP experiment</span>

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References

  1. "MIRACLS". miracls.web.cern.ch. Retrieved 2023-08-02.
  2. Neugart, R; Billowes, J; Bissell, M L; Blaum, K; Cheal, B; Flanagan, K T; Neyens, G; Nörtershäuser, W; Yordanov, D T (2017-06-01). "Collinear laser spectroscopy at ISOLDE: new methods and highlights". Journal of Physics G: Nuclear and Particle Physics. 44 (6): 064002. Bibcode:2017JPhG...44f4002N. doi: 10.1088/1361-6471/aa6642 . ISSN   0954-3899.
  3. Lagaki, V.; Heylen, H.; Belosevic, I.; Fischer, P.; Kanitz, C.; Lechner, S.; Maier, F. M.; Nörtershäuser, W.; Plattner, P.; Rosenbusch, M.; Sels, S.; Schweikhard, L.; Vilen, M.; Wienholtz, F.; Wolf, R. N. (2021-10-21). "An accuracy benchmark of the MIRACLS apparatus: Conventional, single-passage collinear laser spectroscopy inside a MR-ToF device". Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment. 1014: 165663. Bibcode:2021NIMPA101465663L. doi: 10.1016/j.nima.2021.165663 . ISSN   0168-9002.
  4. 1 2 3 4 5 6 Sels, S.; Fischer, P.; Heylen, H.; Lagaki, V.; Lechner, S.; Maier, F. M.; Plattner, P.; Rosenbusch, M.; Wienholtz, F.; Wolf, R. N.; Nörtershäuser, W.; Schweikhard, L.; Malbrunot-Ettenauer, S. (2020-01-15). "First steps in the development of the Multi Ion Reflection Apparatus for Collinear Laser Spectroscopy" (PDF). Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms. 463: 310–314. Bibcode:2020NIMPB.463..310S. doi:10.1016/j.nimb.2019.04.076. ISSN   0168-583X. S2CID   156043276.
  5. Frubose, Clemens Friedrich (26 Sep 2018). "Buffer gas flow simulations for a Paul trap in MIRACLS" (PDF). CERN. Geneva. Department.
  6. 1 2 3 Maier, F. M.; Vilen, M.; Belosevic, I.; Buchinger, F.; Kanitz, C.; Lechner, S.; Leistenschneider, E.; Nörtershäuser, W.; Plattner, P.; Schweikhard, L.; Sels, S.; Wienholtz, F.; Malbrunot-Ettenauer, S. (2023-03-01). "Simulation studies of a 30-keV MR-ToF device for highly sensitive collinear laser spectroscopy". Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment. 1048: 167927. Bibcode:2023NIMPA104867927M. doi: 10.1016/j.nima.2022.167927 . ISSN   0168-9002. S2CID   254957222.
  7. Maier, Franziska Maria (March 2019). "Laser Spectroscopy of Short-Lived- Radionuclides in an Ion Trap: MIRACLS' proof-of-principle experiment and the simulation of the future 30-keV MR-ToF device". Johannes Kepler University Linz.
  8. Lechner, Simon; Fischer, Paul; Heylen, Hanne; Lagaki, Varvara; Maier, Franziska; Plattner, Peter; Rosenbusch, Marco; Sels, Simon; Wienholtz, Frank; Wolf, Robert N.; Nörtershäuser, Wilfried; Schweikhard, Lutz; Malbrunot-Ettenauer, Stephan (2019-08-20). "Fluorescence detection as a new diagnostics tool for electrostatic ion beam traps". Hyperfine Interactions. 240 (1): 1. Bibcode:2019HyInt.240...95L. doi: 10.1007/s10751-019-1628-1 . hdl: 20.500.12708/16264 . ISSN   0304-3843. S2CID   254544306.
  9. Lagaki, V.; Fischer, P.; Heylen, H.; Hummer, F.; Lechner, S.; Sels, S.; Maier, F.; Plattner, P.; Rosenbusch, M.; Wienholtz, F.; Wolf, R.N.; Nörtershäuser, W.; Schweikhard, L.; Malbrunot-Ettenauer, S. (2020). "Stray-light Suppression for the MIRACLS Proof-of-principle Experiment". Acta Physica Polonica B. 51 (3): 571. Bibcode:2020AcPPB..51..571L. doi: 10.5506/APhysPolB.51.571 . ISSN   0587-4254. S2CID   226718972.
  10. Lagaki, Varvara (28 Apr 2021). "Development of an Electrostatic Ion Beam Trap for Laser Spectroscopy of Short-lived Radionuclides" (PDF). PHD: University of Greifswald.