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Light–matter interaction |
---|
Low-energy phenomena: |
Photoelectric effect |
Mid-energy phenomena: |
Thomson scattering |
Compton scattering |
High-energy phenomena: |
Pair production |
Photodisintegration |
Photofission |
Photodisintegration (also called phototransmutation, or a photonuclear reaction) is a nuclear process in which an atomic nucleus absorbs a high-energy gamma ray, enters an excited state, and immediately decays by emitting a subatomic particle. The incoming gamma ray effectively knocks one or more neutrons, protons, or an alpha particle out of the nucleus. [1] The reactions are called (γ,n), (γ,p), and (γ,α).
Photodisintegration is endothermic (energy absorbing) for atomic nuclei lighter than iron and sometimes exothermic (energy releasing) for atomic nuclei heavier than iron. Photodisintegration is responsible for the nucleosynthesis of at least some heavy, proton-rich elements via the p-process in supernovae of type Ib, Ic, or II. This causes the iron to further fuse into the heavier elements.[ citation needed ]
A photon carrying 2.22 MeV or more energy can photodisintegrate an atom of deuterium:
James Chadwick and Maurice Goldhaber used this reaction to measure the proton-neutron mass difference. [2] This experiment proves that a neutron is not a bound state of a proton and an electron,[ why? ] [3] as had been proposed by Ernest Rutherford.
A photon carrying 1.67 MeV or more energy can photodisintegrate an atom of beryllium-9 (100% of natural beryllium, its only stable isotope):
Antimony-124 is assembled with beryllium to make laboratory neutron sources and startup neutron sources. Antimony-124 (half-life 60.20 days) emits β− and 1.690 MeV gamma rays (also 0.602 MeV and 9 fainter emissions from 0.645 to 2.090 MeV), yielding stable tellurium-124. Gamma rays from antimony-124 split beryllium-9 into two alpha particles and a neutron with an average kinetic energy of 24 keV (a so-called intermediate neutron in terms of energy): [4] [5]
Other isotopes have higher thresholds for photoneutron production, as high as 18.72 MeV, for carbon-12. [6]
In explosions of very large stars (250 or more solar masses), photodisintegration is a major factor in the supernova event. As the star reaches the end of its life, it reaches temperatures and pressures where photodisintegration's energy-absorbing effects temporarily reduce pressure and temperature within the star's core. This causes the core to start to collapse as energy is taken away by photodisintegration, and the collapsing core leads to the formation of a black hole. A portion of mass escapes in the form of relativistic jets, which could have "sprayed" the first metals into the universe. [7] [8]
Terrestrial lightnings produce high-speed electrons that create bursts of gamma-rays as bremsstrahlung. The energy of these rays is sometimes sufficient to start photonuclear reactions resulting in emitted neutrons. One such reaction, 14
7N
(γ,n) 13
7N
, is the only natural process other than those induced by cosmic rays in which 13
7N
is produced on Earth. The unstable isotopes remaining from the reaction may subsequently emit positrons by β+ decay. [9]
Photofission is a similar but distinct process, in which a nucleus, after absorbing a gamma ray, undergoes nuclear fission (splits into two fragments of nearly equal mass).
The CNO cycle is one of the two known sets of fusion reactions by which stars convert hydrogen to helium, the other being the proton–proton chain reaction, which is more efficient at the Sun's core temperature. The CNO cycle is hypothesized to be dominant in stars that are more than 1.3 times as massive as the Sun.
The neutron is a subatomic particle, symbol
n
or
n0
, which has no electric charge, and a mass slightly greater than that of a proton. Protons and neutrons constitute the nuclei of atoms. Since protons and neutrons behave similarly within the nucleus, they are both referred to as nucleons. Nucleons have a mass of approximately one atomic mass unit, or dalton. Their properties and interactions are described by nuclear physics. Protons and neutrons are not elementary particles; each is composed of three quarks.
Nuclear fission is a reaction in which the nucleus of an atom splits into two or more smaller nuclei. The fission process often produces gamma photons, and releases a very large amount of energy even by the energetic standards of radioactive decay.
Nucleosynthesis is the process that creates new atomic nuclei from pre-existing nucleons and nuclei. According to current theories, the first nuclei were formed a few minutes after the Big Bang, through nuclear reactions in a process called Big Bang nucleosynthesis. After about 20 minutes, the universe had expanded and cooled to a point at which these high-energy collisions among nucleons ended, so only the fastest and simplest reactions occurred, leaving our universe containing hydrogen and helium. The rest is traces of other elements such as lithium and the hydrogen isotope deuterium. Nucleosynthesis in stars and their explosions later produced the variety of elements and isotopes that we have today, in a process called cosmic chemical evolution. The amounts of total mass in elements heavier than hydrogen and helium remains small, so that the universe still has approximately the same composition.
A neutron source is any device that emits neutrons, irrespective of the mechanism used to produce the neutrons. Neutron sources are used in physics, engineering, medicine, nuclear weapons, petroleum exploration, biology, chemistry, and nuclear power. Neutron source variables include the energy of the neutrons emitted by the source, the rate of neutrons emitted by the source, the size of the source, the cost of owning and maintaining the source, and government regulations related to the source.
In astrophysics, silicon burning is a very brief sequence of nuclear fusion reactions that occur in massive stars with a minimum of about 8–11 solar masses. Silicon burning is the final stage of fusion for massive stars that have run out of the fuels that power them for their long lives in the main sequence on the Hertzsprung–Russell diagram. It follows the previous stages of hydrogen, helium, carbon, neon and oxygen burning processes.
The term p-process (p for proton) is used in two ways in the scientific literature concerning the astrophysical origin of the elements (nucleosynthesis). Originally it referred to a proton capture process which was proposed to be the source of certain, naturally occurring, neutron-deficient isotopes of the elements from selenium to mercury. These nuclides are called p-nuclei and their origin is still not completely understood. Although it was shown that the originally suggested process cannot produce the p-nuclei, later on the term p-process was sometimes used to generally refer to any nucleosynthesis process supposed to be responsible for the p-nuclei.
Neutron emission is a mode of radioactive decay in which one or more neutrons are ejected from a nucleus. It occurs in the most neutron-rich/proton-deficient nuclides, and also from excited states of other nuclides as in photoneutron emission and beta-delayed neutron emission. As only a neutron is lost by this process the number of protons remains unchanged, and an atom does not become an atom of a different element, but a different isotope of the same element.
A radioactive tracer, radiotracer, or radioactive label is a synthetic derivative of a natural compound in which one or more atoms have been replaced by a radionuclide. By virtue of its radioactive decay, it can be used to explore the mechanism of chemical reactions by tracing the path that the radioisotope follows from reactants to products. Radiolabeling or radiotracing is thus the radioactive form of isotopic labeling. In biological contexts, experiments that use radioisotope tracers are sometimes called radioisotope feeding experiments.
In nuclear physics and nuclear chemistry, a nuclear reaction is a process in which two nuclei, or a nucleus and an external subatomic particle, collide to produce one or more new nuclides. Thus, a nuclear reaction must cause a transformation of at least one nuclide to another. If a nucleus interacts with another nucleus or particle, they then separate without changing the nature of any nuclide, the process is simply referred to as a type of nuclear scattering, rather than a nuclear reaction.
Neutron activation is the process in which neutron radiation induces radioactivity in materials, and occurs when atomic nuclei capture free neutrons, becoming heavier and entering excited states. The excited nucleus decays immediately by emitting gamma rays, or particles such as beta particles, alpha particles, fission products, and neutrons. Thus, the process of neutron capture, even after any intermediate decay, often results in the formation of an unstable activation product. Such radioactive nuclei can exhibit half-lives ranging from small fractions of a second to many years.
Neutron capture is a nuclear reaction in which an atomic nucleus and one or more neutrons collide and merge to form a heavier nucleus. Since neutrons have no electric charge, they can enter a nucleus more easily than positively charged protons, which are repelled electrostatically.
Supernova nucleosynthesis is the nucleosynthesis of chemical elements in supernova explosions.
Natural nitrogen (7N) consists of two stable isotopes: the vast majority (99.6%) of naturally occurring nitrogen is nitrogen-14, with the remainder being nitrogen-15. Thirteen radioisotopes are also known, with atomic masses ranging from 9 to 23, along with three nuclear isomers. All of these radioisotopes are short-lived, the longest-lived being nitrogen-13 with a half-life of 9.965(4) min. All of the others have half-lives below 7.15 seconds, with most of these being below 620 milliseconds. Most of the isotopes with atomic mass numbers below 14 decay to isotopes of carbon, while most of the isotopes with masses above 15 decay to isotopes of oxygen. The shortest-lived known isotope is nitrogen-10, with a half-life of 143(36) yoctoseconds, though the half-life of nitrogen-9 has not been measured exactly.
Nuclear astrophysics is an interdisciplinary part of both nuclear physics and astrophysics, involving close collaboration among researchers in various subfields of each of these fields. This includes, notably, nuclear reactions and their rates as they occur in cosmic environments, and modeling of astrophysical objects where these nuclear reactions may occur, but also considerations of cosmic evolution of isotopic and elemental composition (often called chemical evolution). Constraints from observations involve multiple messengers, all across the electromagnetic spectrum (nuclear gamma-rays, X-rays, optical, and radio/sub-mm astronomy), as well as isotopic measurements of solar-system materials such as meteorites and their stardust inclusions, cosmic rays, material deposits on Earth and Moon). Nuclear physics experiments address stability (i.e., lifetimes and masses) for atomic nuclei well beyond the regime of stable nuclides into the realm of radioactive/unstable nuclei, almost to the limits of bound nuclei (the drip lines), and under high density (up to neutron star matter) and high temperature (plasma temperatures up to 109 K). Theories and simulations are essential parts herein, as cosmic nuclear reaction environments cannot be realized, but at best partially approximated by experiments. In general terms, nuclear astrophysics aims to understand the origin of the chemical elements and isotopes, and the role of nuclear energy generation, in cosmic sources such as stars, supernovae, novae, and violent binary-star interactions.
A startup neutron source is a neutron source used for stable and reliable initiation of nuclear chain reaction in nuclear reactors, when they are loaded with fresh nuclear fuel, whose neutron flux from spontaneous fission is insufficient for a reliable startup, or after prolonged shutdown periods. Neutron sources ensure a constant minimal population of neutrons in the reactor core, sufficient for a smooth startup. Without them, the reactor could suffer fast power excursions during startup from state with too few self-generated neutrons.
The nuclear drip line is the boundary beyond which atomic nuclei are unbound with respect to the emission of a proton or neutron.
p-nuclei (p stands for proton-rich) are certain proton-rich, naturally occurring isotopes of some elements between selenium and mercury inclusive which cannot be produced in either the s- or the r-process.
In nuclear physics, properties of a nucleus depend on evenness or oddness of its atomic number Z, neutron number N and, consequently, of their sum, the mass number A. Most importantly, oddness of both Z and N tends to lower the nuclear binding energy, making odd nuclei generally less stable. This effect is not only experimentally observed, but is included in the semi-empirical mass formula and explained by some other nuclear models, such as the nuclear shell model. This difference of nuclear binding energy between neighbouring nuclei, especially of odd-A isobars, has important consequences for beta decay.
The discovery of the neutron and its properties was central to the extraordinary developments in atomic physics in the first half of the 20th century. Early in the century, Ernest Rutherford developed a crude model of the atom, based on the gold foil experiment of Hans Geiger and Ernest Marsden. In this model, atoms had their mass and positive electric charge concentrated in a very small nucleus. By 1920, isotopes of chemical elements had been discovered, the atomic masses had been determined to be (approximately) integer multiples of the mass of the hydrogen atom, and the atomic number had been identified as the charge on the nucleus. Throughout the 1920s, the nucleus was viewed as composed of combinations of protons and electrons, the two elementary particles known at the time, but that model presented several experimental and theoretical contradictions.