| No. | Date | Venue | Opponents | Score | Competition | Brazil scorers | Att. | Ref. |
|---|
| 104 | 6 May 1950 | Pacaembu Stadium, São Paulo (H) | Uruguay | 3–4 | Copa Río Branco | Zizinho, Ademir (2) | — | [1] [3] |
| 105 | 7 May 1950 | Estádio São Januário, Rio de Janeiro (H) | Paraguay | 2–0 | Taça Oswaldo Cruz | Pinga (2) | — | [1] [4] |
| 106 | 13 May 1950 | Pacaembu Stadium, São Paulo (H) | Paraguay | 3–3 | Taça Oswaldo Cruz | Pinga, Maneca, Baltazar | — | [1] [4] |
| 107 | 14 May 1950 | Estádio São Januário, Rio de Janeiro (H) | Uruguay | 3–2 | Copa Río Branco | Ademir, González (o.g.), Chico | — | [1] [3] |
| 108 | 18 May 1950 | Estádio São Januário, Rio de Janeiro (H) | Uruguay | 1–0 | Copa Río Branco | Ademir | — | [1] [3] |
| 109 | 24 June 1950 | Maracanã Stadium, Rio de Janeiro (N) | Mexico | 4–0 | 1950 FIFA World Cup | Ademir (2), Jair, Baltazar | 81,649 | [1] [5] |
| 110 | 28 June 1950 | Pacaembu Stadium, São Paulo (N) | Switzerland | 2–2 | 1950 FIFA World Cup | Alfredo II, Baltazar | 42,032 | [1] [5] |
| 111 | 1 July 1950 | Maracanã Stadium, Rio de Janeiro (N) | Yugoslavia | 2–0 | 1950 FIFA World Cup | Ademir, Zizinho | 142,429 | [1] [5] |
| 112 | 9 July 1950 | Maracanã Stadium, Rio de Janeiro (N) | Sweden | 7–1 | 1950 FIFA World Cup | Ademir (4), Chico (2), Maneca | 138,886 | [1] [5] |
| 113 | 13 July 1950 | Maracanã Stadium, Rio de Janeiro (N) | Spain | 6–1 | 1950 FIFA World Cup | Jair, Chico (2), Ademir, (2), Zizinho | 152,772 | [1] [5] |
| 114 | 16 July 1950 | Maracanã Stadium, Rio de Janeiro (N) | Uruguay | 1–2 | 1950 FIFA World Cup | Friaça | 199,854 | [1] [5] |
| 115 | 6 April 1952 | Estadio Nacional, Santiago (N) | Mexico | 2–0 | 1952 Panamerican Championship | Baltazar (2) | — | [1] [6] |
| 116 | 10 April 1952 | Estadio Nacional, Santiago (N) | Peru | 0–0 | 1952 Panamerican Championship | | — | [1] [6] |
| 117 | 13 April 1952 | Estadio Nacional, Santiago (N) | Panama | 5–0 | 1952 Panamerican Championship | Baltazar, Rodrigues (2), Julinho, Pinga | — | [1] [6] |
| 118 | 16 April 1952 | Estadio Nacional, Santiago (N) | Uruguay | 4–2 | 1952 Panamerican Championship | Didi, Baltazar, Pinga, Rodrigues | — | [1] [6] |
| 119 | 20 April 1952 | Estadio Nacional, Santiago (N) | Chile | 3–0 | 1952 Panamerican Championship | Ademir (2), Pinga | — | [1] [6] |
| 120 | 1 March 1953 | Estadio Nacional, Lima (N) | Bolivia | 8–1 | 1953 South American Championship | Julinho (4), Rodrigues (2), Pinga (2) | 45,000 | [1] [8] |
| 121 | 12 March 1953 | Estadio Nacional, Lima (N) | Ecuador | 2–0 | 1953 South American Championship | Ademir, Cláudio | 35,000 | [1] [8] |
| 122 | 15 March 1953 | Estadio Nacional, Lima (N) | Uruguay | 1–0 | 1953 South American Championship | Ipojucan | 45,000 | [1] [8] |
| 123 | 19 March 1953 | Estadio Nacional, Lima (N) | Peru | 0–1 | 1953 South American Championship | | 55,000 | [1] [8] |
| 124 | 23 March 1953 | Estadio Nacional, Lima (N) | Chile | 3–2 | 1953 South American Championship | Julinho, Zizinho, Baltazar | 35,000 | [1] [8] |
| 125 | 27 March 1953 | Estadio Nacional, Lima (N) | Paraguay | 1–2 | 1953 South American Championship | Nílton Santos | 35,000 | [1] [8] |
| 126 | 1 April 1953 | Estadio Nacional, Lima (N) | Paraguay | 2–3 | 1953 South American Championship | Baltazar (2) | 35,000 | [1] [8] |
| 127 | 28 February 1954 | Estadio Nacional, Santiago (A) | Chile | 2–0 | 1954 FIFA World Cup qualification | Baltazar (2) | — | [1] [9] |
| 128 | 7 March 1954 | Estadio Club Libertad, Asunción (A) | Paraguay | 1–0 | 1954 FIFA World Cup qualification | Baltazar | — | [1] [9] |
| 129 | 14 March 1954 | Maracanã Stadium, Rio de Janeiro (H) | Chile | 1–0 | 1954 FIFA World Cup qualification | Baltazar | — | [1] [9] |
| 130 | 21 March 1954 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 4–1 | 1954 FIFA World Cup qualification | Julinho (2), Baltazar, Maurinho | 174,599 | [1] [9] |
| 131 | 16 June 1954 | Charmilles Stadium, Geneva (N) | Mexico | 5–0 | 1954 FIFA World Cup | Baltazar, Didi, Pinga (2), Julinho | 13,470 | [1] [10] |
| 132 | 19 June 1954 | Stade Olympique de la Pontaise, Lausanne (N) | Yugoslavia | 1–1 ( a.e.t. ) | 1954 FIFA World Cup | Didi | 24,637 | [1] [10] |
| 133 | 27 June 1954 | Wankdorf Stadium, Bern (N) | Hungary | 2–4 | 1954 FIFA World Cup | Djalma Santos, Julinho | 40,000 | [1] [10] |
| 134 | 18 September 1955 | Maracanã Stadium, Rio de Janeiro (H) | Chile | 1–1 | Copa Bernardo O'Higgins | Pinheiro | — | [1] [11] |
| 135 | 20 September 1955 | Pacaembu Stadium, São Paulo (H) | Chile | 2–1 | Copa Bernardo O'Higgins | Maurinho, Álvaro | — | [1] [11] |
| 136 | 13 November 1955 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 3–0 | Taça Oswaldo Cruz | Zizinho (2), Sabará | 65,277 | [1] [4] |
| 137 | 17 November 1955 | Pacaembu Stadium, São Paulo (H) | Paraguay | 3–3 | Taça Oswaldo Cruz | Maurinho, Canhoteiro, Tozzi | 41,478 | [1] [4] |
| 138 | 24 January 1956 | Estadio Centenario, Montevideo (N) | Chile | 1–4 | 1956 South American Championship | Maurinho | 18,000 | [1] [12] |
| 139 | 29 January 1956 | Estadio Centenario, Montevideo (N) | Paraguay | 0–0 | 1956 South American Championship | | 45,000 | [1] [12] |
| 140 | 1 February 1956 | Estadio Centenario, Montevideo (N) | Peru | 2–1 | 1956 South American Championship | Álvaro, Zezinho | 20,000 | [1] [12] |
| 141 | 5 February 1956 | Estadio Centenario, Montevideo (N) | Argentina | 1–0 | 1956 South American Championship | Luizinho | 25,000 | [1] [12] |
| 142 | 10 February 1956 | Estadio Centenario, Montevideo (N) | Uruguay | 0–0 | 1956 South American Championship | | 80,000 | [1] [12] |
| 143 | 1 March 1956 | Estadio Olímpico Universitario, Mexico City (N) | Chile | 2–1 | 1956 Panamerican Championship | Luizinho, Raul Klein | 14,000 | [1] [13] |
| 144 | 6 March 1956 | Estadio Olímpico Universitario, Mexico City (N) | Peru | 1–0 | 1956 Panamerican Championship | Larry | 70,000 | [1] [13] |
| 145 | 8 March 1956 | Estadio Olímpico Universitario, Mexico City (N) | Mexico | 2–1 | 1956 Panamerican Championship | Bodinho, Bravo (o.g.) | 80,000 | [1] [13] |
| 146 | 13 March 1956 | Estadio Olímpico Universitario, Mexico City (N) | Costa Rica | 7–1 | 1956 Panamerican Championship | Larry (3), Chinesinho (3), Bodinho | 65,000 | [1] [13] |
| 147 | 18 March 1956 | Estadio Olímpico Universitario, Mexico City (N) | Argentina | 2–2 | 1956 Panamerican Championship | Chinesinho, Andrade | — | [1] [13] |
| 148 | 8 April 1956 | Estádio Nacional, Lisbon (A) | Portugal | 1–0 | Friendly | Gino | — | [1] |
| 149 | 11 April 1956 | Hardturm, Zürich (A) | Switzerland | 1–1 | Friendly | Gino | — | [1] |
| 150 | 15 April 1956 | Praterstadion, Vienna (A) | Austria | 3–2 | Friendly | Gino, Zózimo, Didi | 65,000 | [1] |
| 151 | 21 April 1956 | Great Strahov Stadium, Prague (A) | Czechoslovakia | 0–0 | Friendly | | 45,000 | [1] |
| 152 | 25 April 1956 | San Siro, Milan (A) | Italy | 0–3 | Friendly | | 80,000 | [1] |
| 153 | 1 May 1956 | Mithatpaşa Stadium, Istanbul (A) | Turkey | 1–0 | Friendly | Djalma Santos | — | [1] |
| 154 | 9 May 1956 | Wembley Stadium, London (A) | England | 2–4 | Friendly | Paulinho, Didi | 97,000 | [1] |
| 155 | 12 June 1956 | Estadio Club Libertad, Asunción (A) | Paraguay | 2–0 | Taça Oswaldo Cruz | Ferreira (2) | — | [1] [4] |
| 156 | 17 June 1956 | Estadio Club Libertad, Asunción (A) | Paraguay | 5–2 | Taça Oswaldo Cruz | Leônidas da Selva, Zizinho (2), Ferreira, Ílton Vaccari | — | [1] [4] |
| 157 | 24 June 1956 | Maracanã Stadium, Rio de Janeiro (H) | Uruguay | 2–0 [A] | Taça do Atlântico | Zizinho, Canário | 59,816 | [1] [14] |
| 158 | 1 July 1956 | Maracanã Stadium, Rio de Janeiro (H) | Italy | 2–0 | Friendly | Ferreira, Canário | 118,514 | [1] |
| 159 | 8 July 1956 | Estadio Presidente Juan Domingo Perón, Avellaneda (A) | Argentina | 0–0 | Taça do Atlântico | | — | [1] [14] |
| 160 | 5 August 1956 | Maracanã Stadium, Rio de Janeiro (H) | Czechoslovakia | 0–1 | Friendly | | 130,000 | [1] |
| 161 | 8 August 1956 | Pacaembu Stadium, São Paulo (H) | Czechoslovakia | 4–1 | Friendly | Zizinho (2), Pepe (2) | 62,000 | [1] |
| 162 | 13 March 1957 | Estadio Nacional, Lima (N) | Chile | 4–2 | 1957 South American Championship | Didi (3), Pepe | 42,000 | [1] [16] |
| 163 | 21 March 1957 | Estadio Nacional, Lima (N) | Ecuador | 7–1 | 1957 South American Championship | Evaristo (3), Pepe, Zizinho, Joel, Didi | 45,000 | [1] [16] |
| 164 | 24 March 1957 | Estadio Nacional, Lima (N) | Colombia | 9–0 | 1957 South American Championship | Pepe, Evaristo (5), Didi (2), Zizinho | 45,000 | [1] [16] |
| 165 | 28 March 1957 | Estadio Nacional, Lima (N) | Uruguay | 2–3 | 1957 South American Championship | Evaristo, Didi | 50,000 | [1] [16] |
| 166 | 31 March 1957 | Estadio Nacional, Lima (N) | Peru | 1–0 [B] | 1957 South American Championship | Didi | 55,000 | [1] [16] |
| 167 | 3 April 1957 | Estadio Nacional, Lima (N) | Argentina | 0–3 | 1957 South American Championship | | 55,000 | [1] [16] |
| 168 | 13 April 1957 | Estadio Nacional, Lima (A) | Peru | 1–1 | 1958 FIFA World Cup qualification | Índio | — | [1] [17] |
| 169 | 21 April 1957 | Maracanã Stadium, Rio de Janeiro (H) | Peru | 1–0 | 1958 FIFA World Cup qualification | Didi | 82,624 | [1] [17] |
| 170 | 11 June 1957 | Maracanã Stadium, Rio de Janeiro (H) | Portugal | 2–1 | Friendly | Didi, Tite | — | [1] |
| 171 | 16 June 1957 | Pacaembu Stadium, São Paulo (H) | Portugal | 3–0 | Friendly | Zito, Mazzola, Del Vecchio | — | [1] |
| 172 | 7 July 1957 | Maracanã Stadium, Rio de Janeiro (H) | Argentina | 1–2 | Copa Julio Argentino Roca | Pelé | — | [1] [18] |
| 173 | 10 July 1957 | Pacaembu Stadium, São Paulo (H) | Argentina | 2–0 ( a.e.t. ) | Copa Julio Argentino Roca | Pelé, Mazzola | — | [1] [18] |
| 174 | 15 September 1957 | Estadio Nacional, Santiago (A) | Chile | 0–1 | Copa Bernardo O'Higgins | | — | [1] [11] |
| 175 | 18 September 1957 | Estadio Nacional, Santiago (A) | Chile | 1–1 ( a.e.t. ) | Copa Bernardo O'Higgins | Matos | — | [1] [11] |
| 176 | 4 May 1958 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 5–1 | Taça Oswaldo Cruz | Zagallo (2), Vavá, Dida, Pelé | — | [1] [4] |
| 177 | 7 May 1958 | Pacaembu Stadium, São Paulo (H) | Paraguay | 0–0 | Taça Oswaldo Cruz | | — | [1] [4] |
| 178 | 14 May 1958 | Maracanã Stadium, Rio de Janeiro (H) | Bulgaria | 4–0 | Friendly | Dida, Moacyr (2), Joel | 140,000 | [1] |
| 179 | 18 May 1958 | Pacaembu Stadium, São Paulo (H) | Bulgaria | 3–1 | Friendly | Pelé (2), Pepe | 70,000 | [1] |
| 180 | 8 June 1958 | Rimnersvallen, Uddevalla (N) | Austria | 3–0 | 1958 FIFA World Cup | Mazzola (2), Nílton Santos | 17,778 | [1] [19] |
| 181 | 11 June 1958 | Ullevi, Gothenburg (N) | England | 0–0 | 1958 FIFA World Cup | | 40,895 | [1] [19] |
| 182 | 15 June 1958 | Ullevi, Gothenburg (N) | Soviet Union | 2–0 | 1958 FIFA World Cup | Vavá (2) | 50,928 | [1] [19] |
| 183 | 19 June 1958 | Ullevi, Gothenburg (N) | Wales | 1–0 | 1958 FIFA World Cup | Pelé | 25,923 | [1] [19] |
| 184 | 24 June 1958 | Råsunda Stadium, Solna (N) | France | 5–2 | 1958 FIFA World Cup | Vavá, Didi, Pelé (3) | 27,100 | [1] [19] |
| 185 | 29 June 1958 | Råsunda Stadium, Solna (N) | Sweden | 5–2 | 1958 FIFA World Cup | Vavá (2), Pelé (2), Zagallo | 49,737 | [1] [19] |
| 186 | 10 March 1959 | Estadio Monumental, Buenos Aires (N) | Peru | 2–2 | 1959 South American Championship (Argentina) | Didi, Pelé | 45,000 | [1] [21] |
| 187 | 15 March 1959 | Estadio Monumental, Buenos Aires (N) | Chile | 3–0 | 1959 South American Championship (Argentina) | Pelé (2), Didi | 40,000 | [1] [21] |
| 188 | 21 March 1959 | Estadio Monumental, Buenos Aires (N) | Bolivia | 4–2 | 1959 South American Championship (Argentina) | Pelé, Paulo Valentim (2), Didi | 25,000 | [1] [21] |
| 189 | 26 March 1959 | Estadio Monumental, Buenos Aires (N) | Uruguay | 3–1 | 1959 South American Championship (Argentina) | Paulo Valentim (3) | 70,000 | [1] [21] |
| 190 | 29 March 1959 | Estadio Monumental, Buenos Aires (N) | Paraguay | 4–1 | 1959 South American Championship (Argentina) | Pelé (3), Chinesinho | 40,000 | [1] [21] |
| 191 | 4 April 1959 | Estadio Monumental, Buenos Aires (N) | Argentina | 1–1 | 1959 South American Championship (Argentina) | Pelé | 85,000 | [1] [21] |
| 192 | 13 May 1959 | Maracanã Stadium, Rio de Janeiro (H) | England | 2–0 | Friendly | Julinho, Henrique Frade | 160,000 | [1] |
| 193 | 17 September 1959 | Maracanã Stadium, Rio de Janeiro (H) | Chile | 7–0 | Copa Bernardo O'Higgins | Pelé (3), Dorval, Quarentinha (2), Dino Sani | — | [1] [11] |
| 194 | 20 September 1959 | Pacaembu Stadium, São Paulo (H) | Chile | 1–0 | Copa Bernardo O'Higgins | Quarentinha | — | [1] [11] |
| 195 | 5 December 1959 | Estadio Modelo, Guayaquil (N) | Paraguay | 3–2 | 1959 South American Championship (Ecuador) | Paulo (3) | 35,000 | [1] [22] |
| 196 | 12 December 1959 | Estadio Modelo, Guayaquil (N) | Uruguay | 0–3 | 1959 South American Championship (Ecuador) | | 55,000 | [1] [22] |
| 197 | 19 December 1959 | Estadio Modelo, Guayaquil (N) | Ecuador | 3–1 | 1959 South American Championship (Ecuador) | Paulo, Geraldo, Zé de Mello | 55,000 | [1] [22] |
| 198 | 22 December 1959 | Estadio Modelo, Guayaquil (N) | Argentina | 1–4 | 1959 South American Championship (Ecuador) | Geraldo | 42,000 | [1] [22] |
| 199 | 27 December 1959 | Estadio Modelo, Guayaquil (A) | Ecuador | 2–1 | Friendly | Traçaia, Zé de Mello | — | [1] |
| 200 | 6 March 1960 | Estadio Nacional, San José (N) | Mexico | 2–2 | 1960 Panamerican Championship | Élton, Gilberto | 30,000 | [1] [23] |
| 201 | 10 March 1960 | Estadio Nacional, San José (N) | Costa Rica | 0–3 | 1960 Panamerican Championship | | — | [1] [23] |
| 202 | 13 March 1960 | Estadio Nacional, San José (N) | Argentina | 1–2 | 1960 Panamerican Championship | Juarez | — | [1] [23] |
| 203 | 15 March 1960 | Estadio Nacional, San José (N) | Mexico | 2–1 | 1960 Panamerican Championship | Alfeu, Mengálvio | 30,000 | [1] [23] |
| 204 | 17 March 1960 | Estadio Nacional, San José (N) | Costa Rica | 4–0 | 1960 Panamerican Championship | Juarez (2), Élton (2) | — | [1] [23] |
| 205 | 20 March 1960 | Estadio Nacional, San José (N) | Argentina | 1–0 | 1960 Panamerican Championship | Mílton Kuelle | — | [1] [23] |
| 206 | 29 April 1960 | Mokhtar El Tetsh Stadium, Cairo (A) | United Arab Republic | 5–0 | Friendly | Quarentinha (2), Garrincha, Pepe (2) | — | [1] |
| 207 | 1 May 1960 | Alexandria Stadium, Alexandria (A) | United Arab Republic | 3–1 | Friendly | Pelé (3) | — | [1] |
| 208 | 6 May 1960 | Mohammed Hassan Helmy Stadium, Cairo (A) | United Arab Republic | 3–0 | Friendly | Quarentinha (2), Garrincha | — | [1] |
| 209 | 26 May 1960 | Estadio Monumental, Buenos Aires (A) | Argentina | 2–4 | Copa Julio Argentino Roca | Djalma Santos, Delém | — | [1] [18] |
| 210 | 29 May 1960 | Estadio Monumental, Buenos Aires (A) | Argentina | 4–1 ( a.e.t. ) | Copa Julio Argentino Roca | Delém (2), Navarro (o.g.), Servílio | 63,500 | [1] [18] |
| 211 | 29 June 1960 | Maracanã Stadium, Rio de Janeiro (H) | Chile | 4–0 | Friendly | Dida, Vavá, Waldo (2) | — | [1] |
| 212 | 3 July 1960 | Estadio Club Libertad, Asunción (A) | Paraguay | 2–1 | Taça do Atlântico | Chinesinho, Delém | — | [1] [14] |
| 213 | 9 July 1960 | Estadio Centenario, Montevideo (A) | Uruguay | 0–1 | Taça do Atlântico | | — | [1] [14] |
| 214 | 12 July 1960 | Maracanã Stadium, Rio de Janeiro (H) | Argentina | 5–1 | Taça do Atlântico | Chinesinho, Pelé, Delém, Pepe (2) | — | [1] [14] |
| 215 | 30 April 1961 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 2–0 | Taça Oswaldo Cruz | Coutinho, Pepe | — | [1] [4] |
| 216 | 3 May 1961 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 3–2 | Taça Oswaldo Cruz | Coutinho (2), Quarentinha | — | [1] [4] |
| 217 | 7 May 1961 | Estadio Nacional, Santiago (A) | Chile | 2–1 | Copa Bernardo O'Higgins | Garrincha, Didi | — | [1] [11] |
| 218 | 11 May 1961 | Estadio Nacional, Santiago (A) | Chile | 1–0 | Copa Bernardo O'Higgins | Gérson | — | [1] [11] |
| 219 | 19 June 1961 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 3–2 | Friendly | Joel, Dida, Henrique Frade | — | [1] |
| 220 | 21 April 1962 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 6–0 | Taça Oswaldo Cruz | Didi, Pelé, Coutinho, Nílton Santos, Vavá, Garrincha | — | [1] [4] |
| 221 | 24 April 1962 | Pacaembu Stadium, São Paulo (H) | Paraguay | 4–0 | Taça Oswaldo Cruz | Pepe, Pelé (2), Vavá | — | [1] [4] |
| 222 | 6 May 1962 | Pacaembu Stadium, São Paulo (H) | Portugal | 2–1 | Friendly | Vavá, Zequinha | — | [1] |
| 223 | 9 May 1962 | Maracanã Stadium, Rio de Janeiro (H) | Portugal | 1–0 | Friendly | Pelé | — | [1] |
| 224 | 12 May 1962 | Maracanã Stadium, Rio de Janeiro (H) | Wales | 3–1 | Friendly | Garrincha, Coutinho, Pelé | — | [1] |
| 225 | 16 May 1962 | Pacaembu Stadium, São Paulo (H) | Wales | 3–1 | Friendly | Vavá, Pelé (2) | — | [1] |
| 226 | 30 May 1962 | Estadio Sausalito, Viña del Mar (N) | Mexico | 2–0 | 1962 FIFA World Cup | Zagallo, Pelé | 10,484 | [1] [25] |
| 227 | 2 June 1962 | Estadio Sausalito, Viña del Mar (N) | Czechoslovakia | 0–0 | 1962 FIFA World Cup | | 14,903 | [1] [25] |
| 228 | 6 June 1962 | Estadio Sausalito, Viña del Mar (N) | Spain | 2–1 | 1962 FIFA World Cup | Amarildo (2) | 18,715 | [1] [25] |
| 229 | 10 June 1962 | Estadio Sausalito, Viña del Mar (N) | England | 3–1 | 1962 FIFA World Cup | Garrincha (2), Vavá | 17,736 | [1] [25] |
| 230 | 13 June 1962 | Estadio Nacional, Santiago (N) | Chile | 4–2 | 1962 FIFA World Cup | Garrincha (2), Vavá (2) | 76,594 | [1] [25] |
| 231 | 17 June 1962 | Estadio Nacional, Santiago (N) | Czechoslovakia | 3–1 | 1962 FIFA World Cup | Amarildo, Zito, Vavá | 68,679 | [1] [25] |
| 232 | 3 March 1963 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 2–2 | Friendly | Flávio, Ilton Chaves | — | [1] |
| 233 | 10 March 1963 | Estadio Félix Capriles, Cochabamba (N) | Peru | 1–0 | 1963 South American Championship | Oswaldo | 18,000 | [1] [26] |
| 234 | 14 March 1963 | Estadio Hernando Siles, La Paz (N) | Colombia | 5–1 | 1963 South American Championship | Flávio, Oswaldo, Marco Antônio, Fernando (2) | 15,000 | [1] [26] |
| 235 | 17 March 1963 | Estadio Hernando Siles, La Paz (N) | Paraguay | 0–2 | 1963 South American Championship | | 8,000 | [1] [26] |
| 236 | 24 March 1963 | Estadio Hernando Siles, La Paz (N) | Argentina | 0–3 | 1963 South American Championship | | 30,000 | [1] [26] |
| 237 | 27 March 1963 | Estadio Félix Capriles, Cochabamba (N) | Ecuador | 2–2 | 1963 South American Championship | Oswaldo (2) | 20,000 | [1] [26] |
| 238 | 31 March 1963 | Estadio Félix Capriles, Cochabamba (N) | Bolivia | 4–5 | 1963 South American Championship | Flávio (2), Marco Antônio, Almir | 25,000 | [1] [26] |
| 239 | 13 April 1963 | Estádio do Morumbi, São Paulo (H) | Argentina | 2–3 | Copa Julio Argentino Roca | Pepe (2) | — | [1] [18] |
| 240 | 16 April 1963 | Maracanã Stadium, Rio de Janeiro (H) | Argentina | 5–2 ( a.e.t. ) | Copa Julio Argentino Roca | Pelé (3), Amarildo (2) | — | [1] [18] |
| 241 | 21 April 1963 | Estádio Nacional, Lisbon (A) | Portugal | 0–1 | Friendly | | — | [1] |
| 242 | 24 April 1963 | Heysel Stadium, Brussels (A) | Belgium | 1–5 | Friendly | Quarentinha | 46,909 | [1] |
| 243 | 28 April 1963 | Stade Olympique de Colombes, Paris (A) | France | 3–2 | Friendly | Pelé (3) | 50,000 | [1] |
| 244 | 2 May 1963 | Olympic Stadium, Amsterdam (A) | Netherlands | 0–1 | Friendly | | 60,000 | [1] |
| 245 | 5 May 1963 | Volksparkstadion, Hamburg (A) | West Germany | 2–1 | Friendly | Coutinho, Pelé | — | [1] |
| 246 | 8 May 1963 | Wembley Stadium, London (A) | England | 1–1 | Friendly | Pepe | 92,000 | [1] |
| 247 | 12 May 1963 | San Siro, Milan (A) | Italy | 0–3 | Friendly | | 72,000 | [1] |
| 248 | 17 May 1963 | Nasser Stadium, Cairo (A) | Egypt | 1–0 | Friendly | Quarentinha | — | [1] |
| 249 | 19 May 1963 | Ramat Gan Stadium, Ramat Gan (A) | Israel | 5–0 | Friendly | Zequinha, Quarentinha (2), Amarildo (2) | 42,000 | [1] |
| 250 | 30 May 1964 | Maracanã Stadium, Rio de Janeiro (H) | England | 5–1 | Taça das Nações | Rinaldo (2), Pelé, Julinho, Roberto Dias | 77,000 | [1] [28] |
| 251 | 3 June 1964 | Pacaembu Stadium, São Paulo (H) | Argentina | 0–3 | Taça das Nações | | 60,000 | [1] [28] |
| 252 | 7 June 1964 | Maracanã Stadium, Rio de Janeiro (H) | Portugal | 4–1 | Taça das Nações | Pelé, Jairzinho, Gérson (2) | 60,000 | [1] [28] |
| 253 | 2 June 1965 | Maracanã Stadium, Rio de Janeiro (H) | Belgium | 5–0 | Friendly | Pelé (3), Flávio, Rinaldo | 110,000 | [1] |
| 254 | 6 June 1965 | Maracanã Stadium, Rio de Janeiro (H) | West Germany | 2–0 | Friendly | Flávio, Pelé | — | [1] |
| 255 | 9 June 1965 | Maracanã Stadium, Rio de Janeiro (H) | Argentina | 0–0 | Friendly | | — | [1] |
| 256 | 17 June 1965 | Parc Municipal, Oran (A) | Algeria | 3–0 | Friendly | Pelé, Dudu, Gérson | — | [1] |
| 257 | 24 June 1965 | Estádio das Antas, Porto (A) | Portugal | 0–0 | Friendly | | — | [1] |
| 258 | 30 June 1965 | Råsunda Stadium, Solna (N) | Sweden | 2–1 | Friendly | Pelé, Gérson | 16,750 | [1] |
| 259 | 4 July 1965 | Central Lenin Stadium, Moscow (A) | Soviet Union | 3–0 | Friendly | Pelé (2), Flávio | 103,000 | [1] |
| 260 | 7 September 1965 | Mineirão, Belo Horizonte (H) | Uruguay | 3–0 | Friendly | Rinaldo, Tupãzinho, Germano | — | [1] |
| 261 | 21 November 1965 | Maracanã Stadium, Rio de Janeiro (H) | Soviet Union | 2–2 | Friendly | Gérson, Pelé | 123,000 | [1] |
| 262 | 17 April 1966 | Estadio Nacional, Santiago (A) | Chile | 1–0 | Copa Bernardo O'Higgins | João Severiano | — | [1] [11] |
| 263 | 20 April 1966 | Estadio Sausalito, Viña del Mar (A) | Chile | 1–2 | Copa Bernardo O'Higgins | João Severiano | — | [1] [11] |
| 264 | 14 May 1966 | Maracanã Stadium, Rio de Janeiro (H) | Wales | 3–1 | Friendly | Silva, Servílio, Garrincha | 64,000 | [1] |
| 265 | 15 May 1966 | Estádio do Morumbi, São Paulo (H) | Chile | 1–1 | Friendly | Rinaldo | — | [1] |
| 266 | 18 May 1966 | Mineirão, Belo Horizonte (H) | Wales | 1–0 | Friendly | Lima | — | [1] |
| 267 | 19 May 1966 | Maracanã Stadium, Rio de Janeiro (H) | Chile | 1–0 | Friendly | Gérson | — | [1] |
| 268 | 4 June 1966 | Estádio do Morumbi, São Paulo (H) | Peru | 4–0 | Friendly | Lima (2), Pelé, Paraná | 16,000 | [1] |
| 269 | 5 June 1966 | Mineirão, Belo Horizonte (H) | Poland | 4–1 | Friendly | Alcindo, Tostão (2), Denílson | — | [1] |
| 270 | 8 June 1966 | Maracanã Stadium, Rio de Janeiro (H) | Peru | 3–1 | Friendly | Fidélis, Tostão, Edu | — | [1] |
| 271 | 8 June 1966 | Maracanã Stadium, Rio de Janeiro (H) | Poland | 2–1 | Friendly | Silva, Garrincha | 109,380 | [1] |
| 272 | 12 June 1966 | Maracanã Stadium, Rio de Janeiro (H) | Czechoslovakia | 2–1 | Friendly | Pelé (2) | 82,976 | [1] |
| 273 | 15 June 1966 | Maracanã Stadium, Rio de Janeiro (H) | Czechoslovakia | 2–2 | Friendly | Pelé, Zito | 62,000 | [1] |
| 274 | 25 June 1966 | Hampden Park, Glasgow (A) | Scotland | 1–1 | Friendly | Servílio | 74,933 | [1] |
| 275 | 30 June 1966 | Ullevi, Gothenburg (A) | Sweden | 3–2 | Friendly | Tostão (2), Gérson | 46,824 | [1] |
| 276 | 12 July 1966 | Goodison Park, Liverpool (N) | Bulgaria | 2–0 | 1966 FIFA World Cup | Pelé, Garrincha | 47,308 | [1] [29] |
| 277 | 15 July 1966 | Goodison Park, Liverpool (N) | Hungary | 1–3 | 1966 FIFA World Cup | Tostão | 51,387 | [1] [29] |
| 278 | 19 July 1966 | Goodison Park, Liverpool (N) | Portugal | 1–3 | 1966 FIFA World Cup | Rildo | 58,479 | [1] [29] |
| 279 | 25 June 1967 | Estadio Centenario, Montevideo (A) | Uruguay | 0–0 | Copa Río Branco | | — | [1] [3] |
| 280 | 28 June 1967 | Estadio Centenario, Montevideo (A) | Uruguay | 2–2 | Copa Río Branco | Paulo Borges (2) | — | [1] [3] |
| 281 | 1 July 1967 | Estadio Centenario, Montevideo (A) | Uruguay | 1–1 | Copa Río Branco | Dirceu Lopes | — | [1] [3] |
| 282 | 19 September 1967 | Estadio Nacional, Santiago (A) | Chile | 1–0 | Friendly | Roberto | — | [1] |
| 283 | 9 June 1968 | Pacaembu Stadium, São Paulo (H) | Uruguay | 2–0 | Copa Río Branco | Tostão, Sadi | — | [1] [3] |
| 284 | 12 June 1968 | Maracanã Stadium, Rio de Janeiro (H) | Uruguay | 4–0 | Copa Río Branco | Paulo Borges, Tostão, Gérson, Jairzinho | — | [1] [3] |
| 285 | 16 June 1968 | Neckarstadion, Stuttgart (A) | West Germany | 1–2 | Friendly | Tostão | 74,164 | [1] |
| 286 | 20 June 1968 | Stadion Dziesięciolecia Manifestu Lipcowego, Warsaw (A) | Poland | 6–3 | Friendly | Natal, Rivellino (2), Tostão, Jairzinho (2) | 51,128 | [1] |
| 287 | 23 June 1968 | Tehelné pole, Bratislava (A) | Czechoslovakia | 2–3 | Friendly | Natal, Carlos Alberto | 60,000 | [1] |
| 288 | 25 June 1968 | JNA Stadium, Belgrade (A) | Yugoslavia | 2–0 | Friendly | Carlos Alberto, Tostão | 30,000 | [1] |
| 289 | 30 June 1968 | Estádio da Machava, Lourenço Marques (N) | Portugal | 2–0 | Friendly | Rivellino, Tostão | 60,000 | [1] |
| 290 | 7 July 1968 | Estadio Azteca, Mexico City (A) | Mexico | 2–0 | Friendly | Jairzinho (2) | — | [1] |
| 291 | 10 July 1968 | Estadio Azteca, Mexico City (A) | Mexico | 1–2 | Friendly | Rivellino | 71,036 | [1] |
| 292 | 14 July 1968 | Estadio Nacional, Lima (A) | Peru | 4–3 | Taça Jorge Chávez/Santos Dumont | Natal, Roberto Miranda, Jairzinho, Carlos Alberto | — | [1] |
| 293 | 17 July 1968 | Estadio Nacional, Lima (A) | Peru | 4–0 | Taça Jorge Chávez/Santos Dumont | Rivellino, Gérson, Tostão, Jairzinho | — | [1] |
| 294 | 25 July 1968 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 4–0 | Taça Oswaldo Cruz | Pelé (2), Toninho Guerreiro, Eduardo | — | [1] |
| 295 | 28 July 1968 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 0–1 | Taça Oswaldo Cruz | | — | [1] |
| 296 | 7 August 1968 | Maracanã Stadium, Rio de Janeiro (H) | Argentina | 4–1 | Friendly | Valtencir, Roberto Miranda (2), Jairzinho | — | [1] [note 1] |
| 297 | 11 August 1968 | Mineirão, Belo Horizonte (H) | Argentina | 3–2 | Friendly | Evaldo, Rodrigues, Dirceu Lopes | — | [1] [note 2] |
| 298 | 31 October 1968 | Maracanã Stadium, Rio de Janeiro (H) | Mexico | 1–2 | Friendly | Carlos Alberto | — | [1] |
| 299 | 3 November 1968 | Mineirão, Belo Horizonte (H) | Mexico | 2–1 | Friendly | Jairzinho, Pelé | — | [1] |
| 300 | 14 December 1968 | Maracanã Stadium, Rio de Janeiro (H) | West Germany | 2–2 | Friendly | Edu (2) | — | [1] |
| 301 | 17 December 1968 | Maracanã Stadium, Rio de Janeiro (H) | Yugoslavia | 3–3 | Friendly | Carlos Alberto, Pelé, Babá | 70,000 | [1] |
| 302 | 19 December 1968 | Mineirão, Belo Horizonte (H) | Yugoslavia | 3–2 | Friendly | Vaguinho, Amauri, Ronaldo | — | [1] |
| 303 | 7 April 1969 | Estádio Beira-Rio, Porto Alegre (H) | Peru | 2–1 | Friendly | Jairzinho, Gérson | — | [1] |
| 304 | 9 April 1969 | Maracanã Stadium, Rio de Janeiro (H) | Peru | 3–2 | Friendly | Pelé, Tostão, Edu | 80,302 | [1] |
| 305 | 12 June 1969 | Maracanã Stadium, Rio de Janeiro (H) | England | 2–1 | Friendly | Tostão, Jairzinho | 135,000 | [1] |
| 306 | 6 August 1969 | Estadio El Campín, Bogotá (A) | Colombia | 2–0 | 1970 FIFA World Cup qualification | Tostão (2) | 51,131 | [1] [40] |
| 307 | 10 August 1969 | Estadio Olímpico, Caracas (A) | Venezuela | 5–0 | 1970 FIFA World Cup qualification | Tostão (3), Pelé (2) | 30,063 | [1] [40] |
| 308 | 17 August 1969 | Estadio Defensores del Chaco, Asunción (A) | Paraguay | 3–0 | 1970 FIFA World Cup qualification | Mendoza (o.g.), Jairzinho, Edu | 44,880 | [1] [40] |
| 309 | 21 August 1969 | Maracanã Stadium, Rio de Janeiro (H) | Colombia | 6–2 | 1970 FIFA World Cup qualification | Tostão (2), Edu, Pelé, Rivellino, Jairzinho | 99,947 | [1] [40] |
| 310 | 24 August 1969 | Maracanã Stadium, Rio de Janeiro (H) | Venezuela | 6–0 | 1970 FIFA World Cup qualification | Tostão (3), Jairzinho, Pelé (2) | 122,841 | [1] [40] |
| 311 | 31 August 1969 | Maracanã Stadium, Rio de Janeiro (H) | Paraguay | 1–0 | 1970 FIFA World Cup qualification | Pelé | 183,341 | [1] [40] |