Breeder reactor

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Assembly of the core of Experimental Breeder Reactor I in Idaho, United States, 1951 Ebr1core.png
Assembly of the core of Experimental Breeder Reactor I in Idaho, United States, 1951

A breeder reactor is a nuclear reactor that generates more fissile material than it consumes. [1] These reactors can be fueled with more-commonly available isotopes of uranium and thorium, such as uranium-238 and thorium-232, as opposed to the rare uranium-235 which is used in conventional reactors. These materials are called fertile materials since they can be bred into fuel by these breeder reactors.

Contents

Breeder reactors achieve this because their neutron economy is high enough to create more fissile fuel than they use. These extra neutrons are absorbed by the fertile material that is loaded into the reactor along with fissile fuel. This irradiated fertile material in turn transmutes into fissile material which can undergo fission reactions.

Breeders were at first found attractive because they made more complete use of uranium fuel than light-water reactors, but interest declined after the 1960s as more uranium reserves were found [2] and new methods of uranium enrichment reduced fuel costs.

Types

Production of heavy transuranic actinides in current thermal-neutron fission reactors through neutron capture and decays. Starting at uranium-238, isotopes of plutonium, americium, and curium are all produced. In a fast neutron-breeder reactor, all these isotopes may be burned as fuel. Sasahara.svg
Production of heavy transuranic actinides in current thermal-neutron fission reactors through neutron capture and decays. Starting at uranium-238, isotopes of plutonium, americium, and curium are all produced. In a fast neutron-breeder reactor, all these isotopes may be burned as fuel.

Many types of breeder reactor are possible:

A "breeder" is simply a nuclear reactor designed for very high neutron economy with an associated conversion rate higher than 1.0. In principle, almost any reactor design could be tweaked to become a breeder. For example, the light-water reactor, a heavily moderated thermal design, evolved into the fast reactor [3] concept, using light water in a low-density supercritical form to increase the neutron economy enough to allow breeding.

Aside from water-cooled, there are many other types of breeder reactor currently envisioned as possible. These include molten-salt cooled, gas cooled, and liquid-metal cooled designs in many variations. Almost any of these basic design types may be fueled by uranium, plutonium, many minor actinides, or thorium, and they may be designed for many different goals, such as creating more fissile fuel, long-term steady-state operation, or active burning of nuclear wastes.

Extant reactor designs are sometimes divided into two broad categories based upon their neutron spectrum, which generally separates those designed to use primarily uranium and transuranics from those designed to use thorium and avoid transuranics. These designs are:

Fast breeder reactor

Schematic diagram showing the difference between the Loop and Pool types of LMFBR LMFBR schematics2.svg
Schematic diagram showing the difference between the Loop and Pool types of LMFBR

All current large-scale FBR power stations were liquid metal fast breeder reactors (LMFBR) cooled by liquid sodium. These have been of one of two designs: [1] :43

There are only two commercially operating breeder reactors as of 2017: the BN-600 reactor, at 560 MWe, and the BN-800 reactor, at 880 MWe. Both are Russian sodium-cooled reactors. The designs use liquid metal as the primary coolant, to transfer heat from the core to steam used to power the electricity generating turbines. FBRs have been built cooled by liquid metals other than sodium—some early FBRs used mercury; other experimental reactors have used a sodium-potassium alloy. Both have the advantage that they are liquids at room temperature, which is convenient for experimental rigs but less important for pilot or full-scale power stations.

Three of the proposed generation IV reactor types are FBRs: [4]

FBRs usually use a mixed oxide fuel core of up to 20% plutonium dioxide (PuO2) and at least 80% uranium dioxide (UO2). Another fuel option is metal alloys, typically a blend of uranium, plutonium, and zirconium (used because it is "transparent" to neutrons). Enriched uranium can be used on its own.

Many designs surround the reactor core in a blanket of tubes that contain non-fissile uranium-238, which, by capturing fast neutrons from the reaction in the core, converts to fissile plutonium-239 (as is some of the uranium in the core), which is then reprocessed and used as nuclear fuel. Other FBR designs rely on the geometry of the fuel (which also contains uranium-238), arranged to attain sufficient fast neutron capture. The plutonium-239 (or the fissile uranium-235) fissile cross-section is much smaller in a fast spectrum than in a thermal spectrum, as is the ratio between the 239Pu/235U fission cross-section and the 238U absorption cross-section. This increases the concentration of 239Pu/235U needed to sustain a chain reaction, as well as the ratio of breeding to fission. [5] On the other hand, a fast reactor needs no moderator to slow down the neutrons at all, taking advantage of the fast neutrons producing a greater number of neutrons per fission than slow neutrons. For this reason ordinary liquid water, being a moderator and neutron absorber, is an undesirable primary coolant for fast reactors. Because large amounts of water in the core are required to cool the reactor, the yield of neutrons and therefore breeding of 239Pu are strongly affected. Theoretical work has been done on reduced moderation water reactors, which may have a sufficiently fast spectrum to provide a breeding ratio slightly over 1. This would likely result in an unacceptable power derating and high costs in a liquid-water-cooled reactor, but the supercritical water coolant of the supercritical water reactor (SCWR) has sufficient heat capacity to allow adequate cooling with less water, making a fast-spectrum water-cooled reactor a practical possibility. [3]

The type of coolants, temperatures, and fast neutron spectrum puts the fuel cladding material (normally austenitic stainless or ferritic-martensitic steels) under extreme conditions. The understanding of the radiation damage, coolant interactions, stresses, and temperatures are necessary for the safe operation of any reactor core. All materials used to date in sodium-cooled fast reactors have known limits. [6] Oxide dispersion-strengthened alloy steel is viewed as the long-term radiation resistant fuel-cladding material that can overcome the shortcomings of today's material choices.

Integral fast reactor

One design of fast neutron reactor, specifically conceived to address the waste disposal and plutonium issues, was the integral fast reactor (IFR, also known as an integral fast breeder reactor, although the original reactor was designed to not breed a net surplus of fissile material). [7] [8]

To solve the waste disposal problem, the IFR had an on-site electrowinning fuel-reprocessing unit that recycled the uranium and all the transuranics (not just plutonium) via electroplating, leaving just short-half-life fission products in the waste. Some of these fission products could later be separated for industrial or medical uses and the rest sent to a waste repository. The IFR pyroprocessing system uses molten cadmium cathodes and electrorefiners to reprocess metallic fuel directly on-site at the reactor. [9] Such systems co-mingle all the minor actinides with both uranium and plutonium. The systems are compact and self-contained, so that no plutonium-containing material needs to be transported away from the site of the breeder reactor. Breeder reactors incorporating such technology would most likely be designed with breeding ratios very close to 1.00, so that after an initial loading of enriched uranium and/or plutonium fuel, the reactor would then be refueled only with small deliveries of natural uranium. A quantity of natural uranium equivalent to a block about the size of a milk crate delivered once per month would be all the fuel such a 1 gigawatt reactor would need. [10] Such self-contained breeders are currently envisioned as the final self-contained and self-supporting ultimate goal of nuclear reactor designers. [11] [5] The project was canceled in 1994 by United States Secretary of Energy Hazel O'Leary. [12] [13]

Other fast reactors

The graphite core of the Molten Salt Reactor Experiment MSRE Core.JPG
The graphite core of the Molten Salt Reactor Experiment

The first fast reactor built and operated was the Los Alamos Plutonium Fast Reactor ("Clementine") in Los Alamos, NM. [14] Clementine was fueled by Ga-stabilized delta-phase Pu and cooled with mercury. It contained a 'window' of Th-232 in anticipation of breeding experiments, but no reports were made available regarding this feature.

Another proposed fast reactor is a fast molten salt reactor, in which the molten salt's moderating properties are insignificant. This is typically achieved by replacing the light metal fluorides (e.g. LiF, BeF2) in the salt carrier with heavier metal chlorides (e.g., KCl, RbCl, ZrCl4).

Several prototype FBRs have been built, ranging in electrical output from a few light bulbs' equivalent (EBR-I, 1951) to over 1,000  MWe. As of 2006, the technology is not economically competitive to thermal reactor technology, but India, Japan, China, South Korea, and Russia are all committing substantial research funds to further development of fast breeder reactors, anticipating that rising uranium prices will change this in the long term. Germany, in contrast, abandoned the technology due to safety concerns. The SNR-300 fast breeder reactor was finished after 19 years despite cost overruns summing up to a total of 3.6 billion, only to then be abandoned. [15]

Thermal breeder reactor

The Shippingport Reactor, used as a prototype light water breeder for five years beginning in August 1977 Shippingport Reactor.jpg
The Shippingport Reactor, used as a prototype light water breeder for five years beginning in August 1977

The advanced heavy-water reactor is one of the few proposed large-scale uses of thorium. [16] India is developing this technology, motivated by substantial thorium reserves; almost a third of the world's thorium reserves are in India, which lacks significant uranium reserves.

The third and final core of the Shippingport Atomic Power Station 60 MWe reactor was a light water thorium breeder, which began operating in 1977. [17] It used pellets made of thorium dioxide and uranium-233 oxide; initially, the U-233 content of the pellets was 5–6% in the seed region, 1.5–3% in the blanket region, and none in the reflector region. It operated at 236 MWt, generating 60 MWe, and ultimately produced over 2.1 billion kilowatt hours of electricity. After five years, the core was removed and found to contain nearly 1.4% more fissile material than when it was installed, demonstrating that breeding from thorium had occurred. [18] [19]

A liquid fluoride thorium reactor is also planned as a thorium thermal breeder. Liquid-fluoride reactors may have attractive features, such as inherent safety, no need to manufacture fuel rods, and possibly simpler reprocessing of the liquid fuel. This concept was first investigated at the Oak Ridge National Laboratory Molten-Salt Reactor Experiment in the 1960s. From 2012 it became the subject of renewed interest worldwide. [20]

Fuel resources

Breeder reactors could, in principle, extract almost all of the energy contained in uranium or thorium, decreasing fuel requirements by a factor of 100 compared to widely used once-through light water reactors, which extract less than 1% of the energy in the actinide metal (uranium or thorium) mined from the earth. [11] The high fuel-efficiency of breeder reactors could greatly reduce concerns about fuel supply, energy used in mining, and storage of radioactive waste. With seawater uranium extraction (currently too expensive to be economical), there is enough fuel for breeder reactors to satisfy the world's energy needs for 5 billion years at 1983's total energy consumption rate, thus making nuclear energy effectively a renewable energy. [21] [22] In addition to seawater, the average crustal granite rocks contain significant quantities of uranium and thorium that with breeder reactors can supply abundant energy for the remaining lifespan of the sun on the main sequence of stellar evolution. [23]

Nuclear waste

Actinides [24] by decay chain Half-life
range (a)
Fission products of 235U by yield [25]
4n 4n + 1 4n + 2 4n + 3 4.5–7%0.04–1.25%<0.001%
228 Ra 4–6 a 155 Euþ
248 Bk [26] > 9 a
244 Cmƒ 241 Puƒ 250 Cf 227 Ac 10–29 a 90 Sr 85 Kr 113m Cdþ
232 Uƒ 238 Puƒ 243 Cmƒ 29–97 a 137 Cs 151 Smþ 121m Sn
249 Cfƒ 242m Amƒ141–351 a

No fission products have a half-life
in the range of 100 a–210 ka ...

241 Amƒ 251 Cfƒ [27] 430–900 a
226 Ra 247 Bk1.3–1.6 ka
240 Pu 229 Th 246 Cmƒ 243 Amƒ4.7–7.4 ka
245 Cmƒ 250 Cm8.3–8.5 ka
239 Puƒ24.1 ka
230 Th 231 Pa32–76 ka
236 Npƒ 233 Uƒ 234 U 150–250 ka 99 Tc 126 Sn
248 Cm 242 Pu 327–375 ka 79 Se
1.33 Ma 135 Cs
237 Npƒ 1.61–6.5 Ma 93 Zr 107 Pd
236 U 247 Cmƒ 15–24 Ma 129 I
244 Pu80 Ma

... nor beyond 15.7 Ma [28]

232 Th 238 U 235 Uƒ№0.7–14.1 Ga

In broad terms, spent nuclear fuel has three main components. The first consists of fission products, the leftover fragments of fuel atoms after they have been split to release energy. Fission products come in dozens of elements and hundreds of isotopes, all of them lighter than uranium. The second main component of spent fuel is transuranics (atoms heavier than uranium), which are generated from uranium or heavier atoms in the fuel when they absorb neutrons but do not undergo fission. All transuranic isotopes fall within the actinide series on the periodic table, and so they are frequently referred to as the actinides. The largest component is the remaining uranium which is around 98.25% uranium-238, 1.1% uranium-235, and 0.65% uranium-236. The U-236 comes from the non-fission capture reaction where U-235 absorbs a neutron but releases only a high energy gamma ray instead of undergoing fission.

The physical behavior of the fission products is markedly different from that of the actinides. In particular, fission products do not undergo fission and therefore cannot be used as nuclear fuel. Indeed, because fission products are often neutron poisons (absorbing neutrons that could be used to sustain a chain reaction), fission products are viewed as nuclear 'ashes' left over from consuming fissile materials. Furthermore, only seven long-lived fission product isotopes have half-lives longer than a hundred years, which makes their geological storage or disposal less problematic than for transuranic materials. [29]

With increased concerns about nuclear waste, breeding fuel cycles came under renewed interest as they can reduce actinide wastes, particularly plutonium and minor actinides. [30] Breeder reactors are designed to fission the actinide wastes as fuel and thus convert them to more fission products. After spent nuclear fuel is removed from a light water reactor, it undergoes a complex decay profile as each nuclide decays at a different rate. There is a large gap in the decay half-lives of fission products compared to transuranic isotopes. If the transuranics are left in the spent fuel, after 1,000 to 100,000 years the slow decay of these transuranics would generate most of the radioactivity in that spent fuel. Thus, removing the transuranics from the waste eliminates much of the long-term radioactivity of spent nuclear fuel. [31]

Today's commercial light-water reactors do breed some new fissile material, mostly in the form of plutonium. Because commercial reactors were never designed as breeders, they do not convert enough uranium-238 into plutonium to replace the uranium-235 consumed. Nonetheless, at least one-third of the power produced by commercial nuclear reactors comes from fission of plutonium generated within the fuel. [32] Even with this level of plutonium consumption, light water reactors consume only part of the plutonium and minor actinides they produce, and nonfissile isotopes of plutonium build up, along with significant quantities of other minor actinides. [33]

Breeding fuel cycles attracted renewed interest because of their potential to reduce actinide wastes, particularly various isotopes of plutonium and the minor actinides (neptunium, americium, curium, etc.). [30] Since breeder reactors on a closed fuel cycle would use nearly all of the isotopes of these actinides fed into them as fuel, their fuel requirements would be reduced by a factor of about 100. The volume of waste they generate would be reduced by a factor of about 100 as well. While there is a huge reduction in the volume of waste from a breeder reactor, the activity of the waste is about the same as that produced by a light-water reactor. [34]

Waste from a breeder reactor has a different decay behavior because it is made up of different materials. Breeder reactor waste is mostly fission products, while light-water reactor waste is mostly unused uranium isotopes and a large quantity of transuranics. After spent nuclear fuel has been removed from a light-water reactor for longer than 100,000 years, the transuranics would be the main source of radioactivity. Eliminating them would eliminate much of the long-term radioactivity from the spent fuel. [31]

In principle, breeder fuel cycles can recycle and consume all actinides, [21] leaving only fission products. As the graphic in this section indicates, fission products have a peculiar "gap" in their aggregate half-lives, such that no fission products have a half-life between 91 and 200,000 years. As a result of this physical oddity, after several hundred years in storage, the activity of the radioactive waste from an FBR would quickly drop to the low level of the long-lived fission products. However, to obtain this benefit requires the highly efficient separation of transuranics from spent fuel. If the fuel reprocessing methods used leave a large fraction of the transuranics in the final waste stream, this advantage would be greatly reduced. [11]

The FBR's fast neutrons can fission actinide nuclei with even numbers of both protons and neutrons. Such nuclei usually lack the low-speed "thermal neutron" resonances of fissile fuels used in LWRs. [35] The thorium fuel cycle inherently produces lower levels of heavy actinides. The fertile material in the thorium fuel cycle has an atomic weight of 232, while the fertile material in the uranium fuel cycle has an atomic weight of 238. That mass difference means that thorium-232 requires six more neutron capture events per nucleus before the transuranic elements can be produced. In addition to this simple mass difference, the reactor gets two chances to fission the nuclei as the mass increases: First as the effective fuel nuclei U233, and as it absorbs two more neutrons, again as the fuel nuclei U235. [36] [37]

A reactor whose main purpose is to destroy actinides rather than increasing fissile fuel-stocks is sometimes known as a burner reactor. Both breeding and burning depend on good neutron economy, and many designs can do either. Breeding designs surround the core by a breeding blanket of fertile material. Waste burners surround the core with non-fertile wastes to be destroyed. Some designs add neutron reflectors or absorbers. [5]

Design

Fission probabilities of selected actinides, thermal vs. fast neutrons. [38] [39] The percentages of thermal and fast fission indicate the fraction of nuclei fissioned when hit by a respective neutron. The remainder undergoes neutron capture.
IsotopeThermal fission
cross section
Thermal
fission
%
Fast fission
cross section
Fast
fission
%
Th-23253.71 microbarn1 n79.94 millibarn3 n
U-23276.52 barn 592.063 barn95
U-233531.3 barn891.908 barn93
U-235585.1 barn811.218 barn80
U-23816.8 microbarn1 n306.4 millibarn11
Np-23720.19 millibarn3 n1.336 barn27
Pu-23817.77 barn71.968 barn70
Pu-239747.4 barn631.802 barn85
Pu-24036.21 millibarn1 n1.328 barn55
Pu-2411012 barn751.626 barn87
Pu-2422.436 millibarn1 n1.151 barn53
Am-2413.122 barn1 n1.395 barn21
Am-242m6401 barn751.834 barn94
Am-24381.58 millibarn1 n1.081 barn23
Cm-2424.665 barn1 n1.775 barn10
Cm-243587.4 barn782.432 barn94
Cm-2441.022 barn4 n1.733 barn33
n=non-fissile

Conversion ratio

One measure of a reactor's performance is the "conversion ratio", defined as the ratio of new fissile atoms produced to fissile atoms consumed. All proposed nuclear reactors except specially designed and operated actinide burners [5] experience some degree of conversion. As long as there is any amount of a fertile material within the neutron flux of the reactor, some new fissile material is always created. When the conversion ratio is greater than 1, it is often called the "breeding ratio".

For example, commonly used light water reactors have a conversion ratio of approximately 0.6. Pressurized heavy-water reactors running on natural uranium have a conversion ratio of 0.8. [40] In a breeder reactor, the conversion ratio is higher than 1. "Break-even" is achieved when the conversion ratio reaches 1.0 and the reactor produces as much fissile material as it uses.

Doubling time

The doubling time is the amount of time it would take for a breeder reactor to produce enough new fissile material to replace the original fuel and additionally produce an equivalent amount of fuel for another nuclear reactor. This was considered an important measure of breeder performance in early years, when uranium was thought to be scarce. However, since uranium is more abundant than thought in the early days of nuclear reactor development, and given the amount of plutonium available in spent reactor fuel, doubling time has become a less important metric in modern breeder-reactor design. [41] [42]

Burnup

"Burnup" is a measure of how much energy has been extracted from a given mass of heavy metal in fuel, often expressed (for power reactors) in terms of gigawatt-days per ton of heavy metal. Burnup is an important factor in determining the types and abundances of isotopes produced by a fission reactor. Breeder reactors by design have high burnup compared to a conventional reactor, as breeder reactors produce more of their waste in the form of fission products, while most or all of the actinides are meant to be fissioned and destroyed. [43]

In the past, breeder-reactor development focused on reactors with low breeding ratios, from 1.01 for the Shippingport Reactor [44] [45] running on thorium fuel and cooled by conventional light water to over 1.2 for the Soviet BN-350 liquid-metal-cooled reactor. [46] Theoretical models of breeders with liquid sodium coolant flowing through tubes inside fuel elements ("tube-in-shell" construction) suggest breeding ratios of at least 1.8 are possible on an industrial scale. [47] The Soviet BR-1 test reactor achieved a breeding ratio of 2.5 under non-commercial conditions. [48]

Reprocessing

Fission of the nuclear fuel in any reactor unavoidably produces neutron-absorbing fission products. The fertile material from a breeder reactor then needs to be reprocessed to remove those neutron poisons. This step is required to fully utilize the ability to breed as much or more fuel than is consumed. All reprocessing can present a proliferation concern, since it can extract weapons-usable material from spent fuel. [49] The most common reprocessing technique, PUREX, presents a particular concern since it was expressly designed to separate plutonium. Early proposals for the breeder-reactor fuel cycle posed an even greater proliferation concern because they would use PUREX to separate plutonium in a highly attractive isotopic form for use in nuclear weapons. [50] [51]

Several countries are developing reprocessing methods that do not separate the plutonium from the other actinides. For instance, the non-water-based pyrometallurgical electrowinning process, when used to reprocess fuel from an integral fast reactor, leaves large amounts of radioactive actinides in the reactor fuel. [11] More conventional water-based reprocessing systems include SANEX, UNEX, DIAMEX, COEX, and TRUEX, and proposals to combine PUREX with those and other co-processes. All these systems have moderately better proliferation resistance than PUREX, though their adoption rate is low. [52] [53] [54]

In the thorium cycle, thorium-232 breeds by converting first to protactinium-233, which then decays to uranium-233. If the protactinium remains in the reactor, small amounts of uranium-232 are also produced, which has the strong gamma emitter thallium-208 in its decay chain. Similar to uranium-fueled designs, the longer the fuel and fertile material remain in the reactor, the more of these undesirable elements build up. In the envisioned commercial thorium reactors, high levels of uranium-232 would be allowed to accumulate, leading to extremely high gamma-radiation doses from any uranium derived from thorium. These gamma rays complicate the safe handling of a weapon and the design of its electronics; this explains why uranium-233 has never been pursued for weapons beyond proof-of-concept demonstrations. [55]

While the thorium cycle may be proliferation-resistant with regard to uranium-233 extraction from fuel (because of the presence of uranium-232), it poses a proliferation risk from an alternate route of uranium-233 extraction, which involves chemically extracting protactinium-233 and allowing it to decay to pure uranium-233 outside of the reactor. This process is an obvious chemical operation which is not required for normal operation of these reactor designs, but it could feasibly happen beyond the oversight of organizations such as the International Atomic Energy Agency (IAEA), and thus must be safeguarded against. [56]

Production

Like many aspects of nuclear power, fast breeder reactors have been subject to much controversy over the years. In 2010 the International Panel on Fissile Materials said "After six decades and the expenditure of the equivalent of tens of billions of dollars, the promise of breeder reactors remains largely unfulfilled and efforts to commercialize them have been steadily cut back in most countries". In Germany, the United Kingdom, and the United States, breeder reactor development programs have been abandoned. [57] [58] The rationale for pursuing breeder reactors—sometimes explicit and sometimes implicit—was based on the following key assumptions: [58] [59]

Some past anti-nuclear advocates have become pro-nuclear power as a clean source of electricity since breeder reactors effectively recycle most of their waste. This solves one of the most-important negative issues of nuclear power. In the documentary Pandora's Promise , a case is made for breeder reactors because they provide a real high-kW alternative to fossil fuel energy. According to the movie, one pound of uranium provides as much energy as 5,000 barrels of oil. [63] [64]

Notable reactors

Notable breeder reactors [14] [65] [66] [67] [68]
ReactorCountry
when built
StartedShut downDesign
MWe
Final
MWe
Thermal
Power MWt
Capacity
factor
Number of
coolant leaks
Neutron
temperature
CoolantReactor class
DFR UK1962197714116534%7Fast NaK Test
China Experimental Fast Reactor China2012operating20226540%8Fast Sodium Test [69]
CFR-600 China2017commissioning/2023642682188234%27Fast Sodium Commercial [70]
BN-350 Soviet Union197319993505275043%15Fast Sodium Prototype
Rapsodie France196719830402FastSodiumTest
Phénix France1975201023313056340.5%31FastSodiumPrototype
PFR UK1976199423423465026.9%20FastSodiumPrototype
KNK IIGermany1977199118175817.1%21FastSodiumResearch/Test
SNR-300 Germany19851991327non-nuclear tests onlyFastSodiumPrototype/Commercial
BN-600 Soviet Union1981operating560560147074.2%27FastSodiumPrototype/Commercial (Gen2)
FFTF US1982199304001FastSodiumTest
Superphénix France198519981200120030007.9%7FastSodiumPrototype/Commercial (Gen2)
FBTR India1985operating13406FastSodiumTest
PFBR India200420245001250FastSodiumPrototype/Commercial (Gen3)
Jōyō Japan197720070150FastSodiumTest
Monju Japan19952017246246714trial only1FastSodiumPrototype
BN-800 Russia2015operating789880210073.4%FastSodiumPrototype/Commercial (Gen3)
MSRE US1965196907.4EpithermalMolten salt (FLiBe)Test
Clementine US1946195200.025Fast Mercury World's First Fast Reactor [14]
EBR-1 US195119640.20.21.4Fast NaK First Power Reactor
Fermi-1 US196319726666200FastSodiumPrototype
EBR-2 US19641994191962.5FastSodiumExperimental/Test
Shippingport US1977
as breeder
19826060236ThermalLight WaterExperimental-Core3

The Soviet Union constructed a series of fast reactors, the first being mercury-cooled and fueled with plutonium metal, and the later plants sodium-cooled and fueled with plutonium oxide. BR-1 (1955) was 100W (thermal) was followed by BR-2 at 100 kW and then the 5 MW BR-5. [48] BOR-60 (first criticality 1969) was 60 MW, with construction started in 1965. [71]

Future plants

The Chinese Experimental Fast Reactor is a 65 MW (thermal), 20 MW (electric), sodium-cooled, pool-type reactor with a 30-year design lifetime and a target burnup of 100 MWd/kg. CEFR (04790005).jpg
The Chinese Experimental Fast Reactor is a 65 MW (thermal), 20 MW (electric), sodium-cooled, pool-type reactor with a 30-year design lifetime and a target burnup of 100 MWd/kg.

India

India has been trying to develop fast breeder reactors for decades but suffered repeated delays. [72] By December 2024 the Prototype Fast Breeder Reactor is due to be completed and commissioned. [73] [74] [75] The program is intended to use fertile thorium-232 to breed fissile uranium-233. India is also pursuing thorium thermal breeder reactor technology. India's focus on thorium is due to the nation's large reserves, though known worldwide reserves of thorium are four times those of uranium. India's Department of Atomic Energy said in 2007 that it would simultaneously construct four more breeder reactors of 500 MWe each including two at Kalpakkam. [76] [ needs update ]

BHAVINI, an Indian nuclear power company, was established in 2003 to construct, commission, and operate all stage II fast breeder reactors outlined in India's three-stage nuclear power programme. To advance these plans, the FBR-600 is a pool-type sodium-cooled reactor with a rating of 600 MWe. [77] [78] [75]

China

The China Experimental Fast Reactor is a 25 MW(e) prototype for the planned China Prototype Fast Reactor. [79] It started generating power in 2011. [80] China initiated a research and development project in thorium molten-salt thermal breeder-reactor technology (liquid fluoride thorium reactor), formally announced at the Chinese Academy of Sciences annual conference in 2011. Its ultimate target was to investigate and develop a thorium-based molten salt nuclear system over about 20 years. [81] [82] [ needs update ]

South Korea

South Korea is developing a design for a standardized modular FBR for export, to complement the standardized pressurized water reactor and CANDU designs they have already developed and built, but has not yet committed to building a prototype.

A cutaway model of the BN-600 reactor, superseded by the BN-800 reactor family BN-600 nuclear reactor.jpg
A cutaway model of the BN-600 reactor, superseded by the BN-800 reactor family
Construction of the BN-800 reactor BN-800 construction.jpg
Construction of the BN-800 reactor

Russia

Russia has a plan for increasing its fleet of fast breeder reactors significantly. A BN-800 reactor (800 MWe) at Beloyarsk was completed in 2012, succeeding a smaller BN-600. [83] It reached its full power production in 2016. [84] Plans for the construction of a larger BN-1200 reactor (1,200 MWe) was scheduled for completion in 2018, with two additional BN-1200 reactors built by the end of 2030. [85] However, in 2015 Rosenergoatom postponed construction indefinitely to allow fuel design to be improved after more experience of operating the BN-800 reactor, and among cost concerns. [86]

An experimental lead-cooled fast reactor, BREST-300 will be built at the Siberian Chemical Combine in Seversk. The BREST (Russian : bystry reaktor so svintsovym teplonositelem, English: fast reactor with lead coolant) design is seen as a successor to the BN series and the 300 MWe unit at the SCC could be the forerunner to a 1,200 MWe version for wide deployment as a commercial power generation unit. The development program is as part of an Advanced Nuclear Technologies Federal Program 2010–2020 that seeks to exploit fast reactors for uranium efficiency while 'burning' radioactive substances that would otherwise be disposed of as waste. Its core would measure about 2.3 metres in diameter by 1.1 metres in height and contain 16 tonnes of fuel. The unit would be refuelled every year, with each fuel element spending five years in total within the core. Lead coolant temperature would be around 540 °C, giving a high efficiency of 43%, primary heat production of 700 MWt yielding electrical power of 300 MWe. The operational lifespan of the unit could be 60 years. The design was expected to be completed by NIKIET in 2014 for construction between 2016 and 2020. [87] By the end of 2024 the cooling tower had been built, and the target for starting operation was 2026.[ citation needed ]

Japan

In 2006 the United States, France, and Japan signed an "arrangement" to research and develop sodium-cooled fast reactors in support of the Global Nuclear Energy Partnership. [88] In 2007 the Japanese government selected Mitsubishi Heavy Industries as the "core company in FBR development in Japan". Shortly thereafter, Mitsubishi FBR Systems was launched to develop and eventually sell FBR technology. [89]

The Marcoule Nuclear Site in France, location of the Phenix (on the left) CEA Marcoule Site.jpg
The Marcoule Nuclear Site in France, location of the Phénix (on the left)

France

In 2010 the French government allocated 651.6 million to the Commissariat à l'énergie atomique to finalize the design of ASTRID (Advanced Sodium Technological Reactor for Industrial Demonstration), a 600 MW fourth-generation reactor design to be finalized in 2020. [90] [91] As of 2013 the UK had shown interest in the PRISM reactor and was working in concert with France to develop ASTRID. In 2019, CEA announced this design would not be built before mid-century. [92]

United States

Kirk Sorensen, former NASA scientist and chief nuclear technologist at Teledyne Brown Engineering, has long been a promoter of thorium fuel cycle and particularly liquid fluoride thorium reactors. In 2011, Sorensen founded Flibe Energy, a company aimed to develop 20–50 MW LFTR reactor designs to power military bases. [93] [94] [95] [96]

In October 2010 GE Hitachi Nuclear Energy signed a memorandum of understanding with the operators of the US Department of Energy's Savannah River Site, which should allow the construction of a demonstration plant based on the company's S-PRISM fast breeder reactor prior to the design receiving full Nuclear Regulatory Commission licensing approval. [97] In October 2011 The Independent reported that the UK Nuclear Decommissioning Authority (NDA) and senior advisers within the Department for Energy and Climate Change (DECC) had asked for technical and financial details of PRISM, partly as a means of reducing the country's plutonium stockpile. [98]

The traveling wave reactor proposed in a patent by Intellectual Ventures is a fast breeder reactor designed to not need fuel reprocessing during the decades-long lifetime of the reactor. The breed-burn wave in the TWR design does not move from one end of the reactor to the other but gradually from the inside out. Moreover, as the fuel's composition changes through nuclear transmutation, fuel rods are continually reshuffled within the core to optimize the neutron flux and fuel usage at any given point in time. Thus, instead of letting the wave propagate through the fuel, the fuel itself is moved through a largely stationary burn wave. This is contrary to many media reports, which have popularized the concept as a candle-like reactor with a burn region that moves down a stick of fuel. By replacing a static core configuration with an actively managed "standing wave" or "soliton" core, TerraPower's design avoids the problem of cooling a highly variable burn region. Under this scenario, the reconfiguration of fuel rods is accomplished remotely by robotic devices; the containment vessel remains closed during the procedure, and there is no associated downtime. [99]

See also

Related Research Articles

<span class="mw-page-title-main">Nuclear reactor</span> Device for controlled nuclear reactions

A nuclear reactor is a device used to initiate and control a fission nuclear chain reaction. Nuclear reactors are used at nuclear power plants for electricity generation and in nuclear marine propulsion. When a fissile nucleus like uranium-235 or plutonium-239 absorbs a neutron, it splits into lighter nuclei, releasing energy, gamma radiation, and free neutrons, which can induce further fission in a self-sustaining chain reaction. The process is carefully controlled using control rods and neutron moderators to regulate the number of neutrons that continue the reaction, ensuring the reactor operates safely, although inherent control by means of delayed neutrons also plays an important role in reactor output control. The efficiency of nuclear fuel is much higher than fossil fuels; the 5% enriched uranium used in the newest reactors has an energy density 120,000 times higher than coal.

<span class="mw-page-title-main">Nuclear fuel cycle</span> Process of manufacturing and using nuclear fuel

The nuclear fuel cycle, also called nuclear fuel chain, is the progression of nuclear fuel through a series of differing stages. It consists of steps in the front end, which are the preparation of the fuel, steps in the service period in which the fuel is used during reactor operation, and steps in the back end, which are necessary to safely manage, contain, and either reprocess or dispose of spent nuclear fuel. If spent fuel is not reprocessed, the fuel cycle is referred to as an open fuel cycle ; if the spent fuel is reprocessed, it is referred to as a closed fuel cycle.

<span class="mw-page-title-main">Nuclear reprocessing</span> Chemical operations that separate fissile material from spent fuel to be recycled as new fuel

Nuclear reprocessing is the chemical separation of fission products and actinides from spent nuclear fuel. Originally, reprocessing was used solely to extract plutonium for producing nuclear weapons. With commercialization of nuclear power, the reprocessed plutonium was recycled back into MOX nuclear fuel for thermal reactors. The reprocessed uranium, also known as the spent fuel material, can in principle also be re-used as fuel, but that is only economical when uranium supply is low and prices are high. Nuclear reprocessing may extend beyond fuel and include the reprocessing of other nuclear reactor material, such as Zircaloy cladding.

Mixed oxide fuel, commonly referred to as MOX fuel, is nuclear fuel that contains more than one oxide of fissile material, usually consisting of plutonium blended with natural uranium, reprocessed uranium, or depleted uranium. MOX fuel is an alternative to the low-enriched uranium fuel used in the light-water reactors that predominate nuclear power generation.

<span class="mw-page-title-main">Fast-neutron reactor</span> Nuclear reactor where fast neutrons maintain a fission chain reaction

A fast-neutron reactor (FNR) or fast-spectrum reactor or simply a fast reactor is a category of nuclear reactor in which the fission chain reaction is sustained by fast neutrons, as opposed to slow thermal neutrons used in thermal-neutron reactors. Such a fast reactor needs no neutron moderator, but requires fuel that is relatively rich in fissile material when compared to that required for a thermal-neutron reactor. Around 20 land based fast reactors have been built, accumulating over 400 reactor years of operation globally. The largest was the Superphénix sodium cooled fast reactor in France that was designed to deliver 1,242 MWe. Fast reactors have been studied since the 1950s, as they provide certain advantages over the existing fleet of water-cooled and water-moderated reactors. These are:

In nuclear physics, an energy amplifier is a novel type of nuclear power reactor, a subcritical reactor, in which an energetic particle beam is used to stimulate a reaction, which in turn releases enough energy to power the particle accelerator and leave an energy profit for power generation. The concept has more recently been referred to as an accelerator-driven system (ADS) or accelerator-driven sub-critical reactor.

A subcritical reactor is a nuclear fission reactor concept that produces fission without achieving criticality. Instead of sustaining a chain reaction, a subcritical reactor uses additional neutrons from an outside source. There are two general classes of such devices. One uses neutrons provided by a nuclear fusion machine, a concept known as a fusion–fission hybrid. The other uses neutrons created through spallation of heavy nuclei by charged particles such as protons accelerated by a particle accelerator, a concept known as an accelerator-driven system (ADS) or accelerator-driven sub-critical reactor.

<span class="mw-page-title-main">Integral fast reactor</span> Nuclear reactor design

The integral fast reactor (IFR), originally the advancedliquid-metal reactor (ALMR), is a design for a nuclear reactor using fast neutrons and no neutron moderator. IFRs can breed more fuel and are distinguished by a nuclear fuel cycle that uses reprocessing via electrorefining at the reactor site.

<span class="mw-page-title-main">Bhabha Atomic Research Centre</span> Nuclear research facility in Mumbai, India

The Bhabha Atomic Research Centre (BARC) is India's premier nuclear research facility, headquartered in Trombay, Mumbai, Maharashtra, India. It was founded by Homi Jehangir Bhabha as the Atomic Energy Establishment, Trombay (AEET) in January 1954 as a multidisciplinary research program essential for India's nuclear program. It operates under the Department of Atomic Energy (DAE), which is directly overseen by the Prime Minister of India.

<span class="mw-page-title-main">Fertile material</span> Substance that can be converted into material for use in nuclear fission

Fertile material is a material that, although not fissile itself, can be converted into a fissile material by neutron absorption.

Generation IVreactors are nuclear reactor design technologies that are envisioned as successors of generation III reactors. The Generation IV International Forum (GIF) – an international organization that coordinates the development of generation IV reactors – specifically selected six reactor technologies as candidates for generation IV reactors. The designs target improved safety, sustainability, efficiency, and cost. The World Nuclear Association in 2015 suggested that some might enter commercial operation before 2030.

<span class="mw-page-title-main">Sodium-cooled fast reactor</span> Type of nuclear reactor cooled by molten sodium

A sodium-cooled fast reactor is a fast neutron reactor cooled by liquid sodium.

<span class="mw-page-title-main">Thorium fuel cycle</span> Nuclear fuel cycle

The thorium fuel cycle is a nuclear fuel cycle that uses an isotope of thorium, 232
Th
, as the fertile material. In the reactor, 232
Th
is transmuted into the fissile artificial uranium isotope 233
U
which is the nuclear fuel. Unlike natural uranium, natural thorium contains only trace amounts of fissile material, which are insufficient to initiate a nuclear chain reaction. Additional fissile material or another neutron source is necessary to initiate the fuel cycle. In a thorium-fuelled reactor, 232
Th
absorbs neutrons to produce 233
U
. This parallels the process in uranium breeder reactors whereby fertile 238
U
absorbs neutrons to form fissile 239
Pu
. Depending on the design of the reactor and fuel cycle, the generated 233
U
either fissions in situ or is chemically separated from the used nuclear fuel and formed into new nuclear fuel.

<span class="mw-page-title-main">Spent nuclear fuel</span> Nuclear fuel thats been irradiated in a nuclear reactor

Spent nuclear fuel, occasionally called used nuclear fuel, is nuclear fuel that has been irradiated in a nuclear reactor. It is no longer useful in sustaining a nuclear reaction in an ordinary thermal reactor and, depending on its point along the nuclear fuel cycle, it will have different isotopic constituents than when it started.

In nuclear power technology, burnup is a measure of how much energy is extracted from a primary nuclear fuel source. It is measured as the fraction of fuel atoms that underwent fission in %FIMA or %FIFA as well as, preferably, the actual energy released per mass of initial fuel in gigawatt-days/metric ton of heavy metal (GWd/tHM), or similar units.

The Reduced-Moderation Water Reactor (RMWR), also referred to as the Resource-renewable BWR, is a proposed type of light water moderated nuclear power reactor, featuring some characteristics of a fast neutron reactor, thereby combining the established and proven technology of light water reactors with the desired features of fast neutron reactors. The RMWR concept builds upon the Advanced Boiling Water Reactor and is under active development in theoretical studies, particularly in Japan. Hitachi and the Japan Atomic Energy Agency are both involved in research.

<span class="mw-page-title-main">Liquid fluoride thorium reactor</span> Type of nuclear reactor that uses molten material as fuel

The liquid fluoride thorium reactor is a type of molten salt reactor. LFTRs use the thorium fuel cycle with a fluoride-based molten (liquid) salt for fuel. In a typical design, the liquid is pumped between a critical core and an external heat exchanger where the heat is transferred to a nonradioactive secondary salt. The secondary salt then transfers its heat to a steam turbine or closed-cycle gas turbine.

<span class="mw-page-title-main">Traveling wave reactor</span> Type of nuclear fission reactor

A traveling-wave reactor (TWR) is a proposed type of nuclear fission reactor that can convert fertile material into usable fuel through nuclear transmutation, in tandem with the burnup of fissile material. TWRs differ from other kinds of fast-neutron and breeder reactors in their ability to use fuel efficiently without uranium enrichment or reprocessing, instead directly using depleted uranium, natural uranium, thorium, spent fuel removed from light water reactors, or some combination of these materials. The concept is still in the development stage and no TWRs have ever been built.

Hybrid nuclear fusion–fission is a proposed means of generating power by use of a combination of nuclear fusion and fission processes.

<span class="mw-page-title-main">Nuclear transmutation</span> Conversion of an atom from one element to another

Nuclear transmutation is the conversion of one chemical element or an isotope into another chemical element. Nuclear transmutation occurs in any process where the number of protons or neutrons in the nucleus of an atom is changed.

References

  1. 1 2 Waltar AE, Reynolds AB (1981). Fast breeder reactors. New York: Pergamon Press. ISBN   978-0-08-025983-3. Archived from the original on 5 January 2014. Retrieved 4 June 2016.
  2. Helmreich, J. E. Gathering Rare Ores: The Diplomacy of Uranium Acquisition, 1943–1954, Princeton UP, 1986: ch. 10 ISBN   0-7837-9349-9.
  3. 1 2 T. Nakatsuka; et al. Current Status of Research and Development of Supercritical Water-Cooled Fast Reactor (Super Fast Reactor) in Japan. Presented at IAEA Technical Committee Meeting on SCWRs in Pisa, 5–8 July 2010.
  4. "A Technology Roadmap for Generation IV Nuclear Energy Systems" (PDF). Generation IV International Forum. December 2002. GIF-002-00. Archived (PDF) from the original on 1 July 2015. Retrieved 1 July 2015.
  5. 1 2 3 4 E. A. Hoffman; W. S. Yang; R. N. Hill. "Preliminary Core Design Studies for the Advanced Burner Reactor over a Wide Range of Conversion Ratios" (PDF). Argonne National Laboratory. ANL-AFCI-177.
  6. Davis, Thomas P. (2018). "Review of the iron-based materials applicable for the fuel and core of future Sodium Fast Reactors (SFR)" (PDF). Office for Nuclear Regulation. Archived (PDF) from the original on 3 January 2019. Retrieved 2 January 2019.
  7. "The Integral Fast Reactor". Reactors Designed by Argonne National Laboratory. Argonne National Laboratory. Archived from the original on 17 September 2013. Retrieved 20 May 2013.
  8. "National Policy Analysis #378: Integral Fast Reactors: Source of Safe, Abundant, Non-Polluting Power – December 2001". Archived from the original on 25 January 2016. Retrieved 13 October 2007.
  9. Hannum, W.H., Marsh, G.E., and Stanford, G.S. (2004). PUREX and PYRO are not the same Archived 23 January 2022 at the Wayback Machine . Physics and Society, July 2004.
  10. University of Washington (2004). Energy Numbers: Energy in natural processes and human consumption, some numbers Archived 15 September 2012 at the Wayback Machine . Retrieved 16 October 2007.
  11. 1 2 3 4 "Pyroprocessing Technologies: Recycling Used Nuclear Fuel For A Sustainable Energy Future" (PDF). Argonne National Laboratory. Archived (PDF) from the original on 19 February 2013.
  12. Kirsch, Steve. "The Integral Fast Reactor (IFR) project: Congress Q&A". Archived from the original on 16 December 2012. Retrieved 25 December 2012.
  13. Stanford, George S. "Comments on the Misguided Termination of the IFR Project" (PDF). Archived (PDF) from the original on 15 December 2012. Retrieved 25 December 2012.
  14. 1 2 3 Patenaude, Hannah K.; Freibert, Franz J. (3 July 2023). "Oh, My Darling Clementine: A Detailed History and Data Repository of the Los Alamos Plutonium Fast Reactor". Nuclear Technology. 209 (7): 963–1007. doi: 10.1080/00295450.2023.2176686 . ISSN   0029-5450.
  15. Werner Meyer-Larsen: Der Koloß von Kalkar. Der Spiegel 43/1981 vom 19 October 1981, S. 42–55. [["Der Koloß von Kalkar", Der Spiegel , 13 September]] (German)
  16. "Thorium". Archived from the original on 19 April 2012. Retrieved 14 June 2012.
  17. "Shippingport Atomic Power Station: A National Historic Mechanical Engineering Landmark" (PDF). Archived (PDF) from the original on 29 November 2007.
  18. Adams, Rod (1 October 1995). "Light Water Breeder Reactor: Adapting A Proven System". Archived from the original on 28 October 2012. Retrieved 2 October 2012.
  19. Thorium Archived 19 April 2012 at the Wayback Machine information from the World Nuclear Association
  20. Stenger, Victor (12 January 2012). "LFTR: A Long-Term Energy Solution?". Huffington Post. Archived from the original on 22 December 2016. Retrieved 30 September 2012.
  21. 1 2 Cohen, Bernard L. "Breeder reactors: A renewable energy source" (PDF). Argonne National Laboratory. Archived from the original (PDF) on 14 January 2013. Retrieved 25 December 2012.
  22. Weinberg, A. M., and R. P. Hammond (1970). "Limits to the use of energy," Am. Sci. 58, 412.
  23. "There's Atomic Energy in Granite". 8 February 2013.
  24. Plus radium (element 88). While actually a sub-actinide, it immediately precedes actinium (89) and follows a three-element gap of instability after polonium (84) where no nuclides have half-lives of at least four years (the longest-lived nuclide in the gap is radon-222 with a half life of less than four days). Radium's longest lived isotope, at 1,600 years, thus merits the element's inclusion here.
  25. Specifically from thermal neutron fission of uranium-235, e.g. in a typical nuclear reactor.
  26. Milsted, J.; Friedman, A. M.; Stevens, C. M. (1965). "The alpha half-life of berkelium-247; a new long-lived isomer of berkelium-248". Nuclear Physics. 71 (2): 299. Bibcode:1965NucPh..71..299M. doi:10.1016/0029-5582(65)90719-4.
    "The isotopic analyses disclosed a species of mass 248 in constant abundance in three samples analysed over a period of about 10 months. This was ascribed to an isomer of Bk248 with a half-life greater than 9 [years]. No growth of Cf248 was detected, and a lower limit for the β half-life can be set at about 104 [years]. No alpha activity attributable to the new isomer has been detected; the alpha half-life is probably greater than 300 [years]."
  27. This is the heaviest nuclide with a half-life of at least four years before the "sea of instability".
  28. Excluding those "classically stable" nuclides with half-lives significantly in excess of 232Th; e.g., while 113mCd has a half-life of only fourteen years, that of 113Cd is eight quadrillion years.
  29. "Radioactive Waste Management". World Nuclear Association. Archived from the original on 21 September 2013. Retrieved 19 September 2013.
  30. 1 2 "Supply of Uranium". World Nuclear Association. Archived from the original on 12 February 2013. Retrieved 11 March 2012.
  31. 1 2 Bodansky, David (January 2006). "The Status of Nuclear Waste Disposal". Physics and Society. 35 (1). American Physical Society. Archived from the original on 16 May 2008. Retrieved 30 July 2012.
  32. "Information Paper 15". World Nuclear Association. Archived from the original on 30 March 2010. Retrieved 15 December 2012.
  33. U. Mertyurek; M. W. Francis; I. C. Gauld. "SCALE 5 Analysis of BWR Spent Nuclear Fuel Isotopic Compositions for Safety Studies" (PDF). ORNL/TM-2010/286. OAK RIDGE NATIONAL LABORATORY. Archived (PDF) from the original on 17 February 2013. Retrieved 25 December 2012.
  34. "Fast Breeder Reactors" (PDF). Archived (PDF) from the original on 29 March 2016. Retrieved 4 June 2016.
  35. "Neutron Cross Sections4.7.2". National Physical Laboratory. Archived from the original on 1 January 2013. Retrieved 17 December 2012.
  36. David, Sylvain; Elisabeth Huffer; Hervé Nifenecker. "Revisiting the thorium-uranium nuclear fuel cycle" (PDF). europhysicsnews. Archived from the original (PDF) on 12 July 2007. Retrieved 11 November 2018.
  37. "Fissionable Isotopes". Archived from the original on 8 November 2012. Retrieved 25 December 2012.
  38. "Plentiful Energy: The Story of the Integral Fast Reactor" (PDF). p. 21. Archived (PDF) from the original on 27 October 2014. Retrieved 2 March 2015.
  39. "Cross Section Table".
  40. Kadak, Prof. Andrew C. "Lecture 4, Fuel Depletion & Related Effects". Operational Reactor Safety 22.091/22.903. Hemisphere, as referenced by MIT. p. Table 6–1, "Average Conversion or Breeding Ratios for Reference Reactor Systems". Archived from the original on 17 October 2015. Retrieved 24 December 2012.
  41. Rodriguez, Placid; Lee, S. M. "Who is afraid of breeders?". Indira Gandhi Centre for Atomic Research, Kalpakkam 603 102, India. Archived from the original on 26 March 2013. Retrieved 24 December 2012.
  42. R. Prasad (10 October 2002). "Fast breeder reactor: Is advanced fuel necessary?". The Hindu . Chennai, India. Archived from the original on 5 December 2003.
  43. "Fast Reactor Systems and Innovative Fuels for Minor Actinides Homogeneous Recycling" (PDF). Archived (PDF) from the original on 13 October 2016.
  44. Adams, R. (1995). Light Water Breeder Reactor (Archived 15 September 2007 at the Wayback Machine ), Atomic Energy Insights1.
  45. Kasten, P. R. (1998) Review of the Radkowsky Thorium Reactor Concept (Archived 25 February 2009 at the Wayback Machine ). Science & Global Security7, 237–269.
  46. Fast Breeder Reactors (Archived 11 September 2006 at the Wayback Machine ), Department of Physics & Astronomy, Georgia State University. Retrieved 16 October 2007.
  47. Hiraoka, T., Sako, K., Takano, H., Ishii, T., and Sato, M. (1991). A high-breeding fast reactor with fission product gas purge/tube-in-shell metallic fuel assemblies (Archived 29 September 2007 at the Wayback Machine ). Nuclear Technology93, 305–329.
  48. 1 2 Valerii Korobeinikov (31 March – 2 April 2014). Innovative Concepts Based on Fast Reactor Technology (PDF). 1st Consultancy Meeting for Review of Innovative Reactor Concepts for Prevention of Severe Accidents and Mitigation of their Consequences. International Atomic Energy Agency. Archived from the original (PDF) on 4 March 2016.
  49. R. Bari; et al. (2009). "Proliferation Risk Reduction Study ofAlternative Spent Fuel Processing" (PDF). BNL-90264-2009-CP. Brookhaven National Laboratory. Archived (PDF) from the original on 21 September 2013. Retrieved 16 December 2012.
  50. C.G. Bathke; et al. (2008). "An Assessment of the Proliferation Resistance of Materials in Advanced Fuel Cycles" (PDF). Department of Energy. Archived from the original (PDF) on 4 June 2009. Retrieved 16 December 2012.
  51. "An Assessment of the Proliferation Resistance of Materials in Advanced Nuclear Fuel Cycles" (PDF). 2008. Archived from the original (PDF) on 21 September 2013. Retrieved 16 December 2012.
  52. Ozawa, M.; Sano, Y.; Nomura, K.; Koma, Y.; Takanashi, M. "A New Reprocessing System Composed of PUREX and TRUEX Processes For Total Separation of Long-lived Radionuclides" (PDF). Archived (PDF) from the original on 21 September 2013. Retrieved 20 September 2013.
  53. Simpson, Michael F.; Law, Jack D. (February 2010). "Nuclear Fuel Reprocessing" (PDF). Idaho National Laboratory. Archived (PDF) from the original on 21 September 2013. Retrieved 20 September 2013.
  54. "Proliferation Risk Reduction Study of Alternative Spent Fuel Processing" (PDF). Archived (PDF) from the original on 1 January 2017. Retrieved 1 January 2017.
  55. Kang and Von Hippel (2001). "U-232 and the Proliferation-Resistance of U-233 in Spent Fuel" (PDF). 0892-9882/01. Science & Global Security, Volume 9 pp 1–32. Archived from the original (PDF) on 30 March 2015. Retrieved 18 December 2012.
  56. "Thorium: Proliferation warnings on nuclear 'wonder-fuel'". 2012. Archived from the original on 23 September 2017. Retrieved 22 September 2017.
  57. M.V. Ramana; Mycle Schneider (May–June 2010). "It's time to give up on breeder reactors" (PDF). Bulletin of the Atomic Scientists . Archived (PDF) from the original on 6 December 2013. Retrieved 3 December 2013.
  58. 1 2 Frank von Hippel; et al. (February 2010). Fast Breeder Reactor Programs: History and Status (PDF). International Panel on Fissile Materials. ISBN   978-0-9819275-6-5. Archived (PDF) from the original on 7 April 2020. Retrieved 28 April 2014.
  59. M.V. Ramana; Mycle Schneider (May–June 2010). "It's time to give up on breeder reactors" (PDF). Bulletin of the Atomic Scientists. Archived (PDF) from the original on 6 December 2013. Retrieved 3 December 2013.
  60. "Global Uranium Supply and Demand – Council on Foreign Relations". Archived from the original on 10 April 2012. Retrieved 10 February 2012.
  61. "Global Uranium Supply and Demand – Council on Foreign Relations". Archived from the original on 5 May 2012. Retrieved 25 July 2012.
  62. Introduction to Weapons of Mass Destruction, Langford, R. Everett (2004). Hoboken, New Jersey: John Wiley & Sons. p. 85. ISBN   0-471-46560-7. "The US tested a few uranium-233 bombs, but the presence of uranium-232 in the uranium-233 was a problem; the uranium-232 is a copious alpha emitter and tended to 'poison' the uranium-233 bomb by knocking stray neutrons from impurities in the bomb material, leading to possible pre-detonation. Separation of the uranium-232 from the uranium-233 proved to be very difficult and not practical. The uranium-233 bomb was never deployed since plutonium-239 was becoming plentiful."
  63. Len Koch, pioneering nuclear engineer (2013). Pandora's Promise (Motion picture). Impact Partners and CNN Films. 11 minutes in. Archived from the original (DVD, streaming) on 18 April 2014. Retrieved 24 April 2014. One pound of uranium, which is the size of my fingertip, if you could release all of the energy, has the equivalent of about 5,000 barrels of oil.
  64. Len Koch (2013). Pandora's Promise. Netflix (Motion picture).[ permanent dead link ]
  65. "Nuclear Fusion: WNA - World Nuclear Association". Archived from the original on 16 March 2015. Retrieved 2 March 2015.
  66. S. R. Pillai, M. V. Ramana (2014). "Breeder reactors: A possible connection between metal corrosion and sodium leaks". Bulletin of the Atomic Scientists. 70 (3): 49–55. Bibcode:2014BuAtS..70c..49P. doi:10.1177/0096340214531178. S2CID   144406710. Archived from the original on 17 October 2015. Retrieved 15 February 2015.
  67. "Database on Nuclear Power Reactors". PRIS. IAEA. Archived from the original on 2 June 2013. Retrieved 15 February 2015.
  68. "Experimental Breeder Reactor 1 (EBR-1) - Cheeka Tales". Archived from the original on 2 April 2015. Retrieved 2 March 2015.
  69. "Chinese fast reactor begins high-power operation: New Nuclear - World Nuclear News".
  70. "China's New Breeder Reactors May Produce More Than Just Watts - IEEE Spectrum".
  71. FSUE "State Scientific Center of Russian Federation Research Institute of Atomic Reactors". "Experimental fast reactor BOR-60". Archived from the original on 31 December 2012. Retrieved 15 June 2012.
  72. "India's First Prototype Fast Breeder Reactor Has a New Deadline. Should We Trust It? – the Wire Science". 20 August 2020.
  73. Srikanth (27 November 2011). "80% of work on fast breeder reactor at Kalpakkam over". The Hindu. Kalpakkam. Archived from the original on 28 November 2011. Retrieved 25 March 2012.
  74. Jaganathan, Venkatachari (11 May 2011). "India's new fast-breeder on track, nuclear power from September next". Hindustan Times. Chennai. Archived from the original on 13 May 2013. Retrieved 25 March 2012.
  75. 1 2 "India's first Prototype Fast Breeder Reactor in final stages of commissioning". The New Indian Express. Archived from the original on 20 September 2021. Retrieved 20 September 2021.
  76. "Home – India Defence". Archived from the original on 24 November 2011.
  77. Conceptual Design of PFBR Core S.M. Lee, S Govindarajan, R. Indira, T.M. John, P. Mohanakrishnan, R. Shankar Singh, S B. Bhoje Indira Gandhi Centre for Atomic Research (IGCAR), Kalpakkam, India https://inis.iaea.org/collection/NCLCollectionStore/_Public/28/014/28014318.pdf Archived 20 September 2021 at the Wayback Machine
  78. "FBR-600 - India's Next-gen Commercial Fast Breeder Reactor [CFBR]". Archived from the original on 20 September 2021. Retrieved 20 September 2021.
  79. "IAEA Fast Reactor Database" (PDF). Archived (PDF) from the original on 28 June 2011. Retrieved 13 March 2011.
  80. "China's experimental fast neutron reactor begins generating power". xinhuanet. July 2011. Archived from the original on 7 April 2016. Retrieved 21 July 2011.
  81. Qimin, Xu (26 January 2011). "The future of nuclear power plant safety "are not picky eaters"" (in Chinese). Archived from the original on 17 July 2012. Retrieved 30 October 2011. Yesterday, as the Chinese Academy of Sciences of the first to start one of the strategic leader in science and technology projects, "the future of advanced nuclear fission energy – nuclear energy, thorium-based molten salt reactor system" project was officially launched. The scientific goal is 20 years or so, developed a new generation of nuclear energy systems, all the technical level reached in the test and have all the intellectual property rights.
  82. Clark, Duncan (16 February 2011). "China enters race to develop nuclear energy from thorium". Environment Blog. London: The Guardian (UK). Archived from the original on 19 May 2017. Retrieved 30 October 2011.
  83. "Белоярская АЭС: начался выход БН-800 на минимальный уровень мощности". AtomInfo.ru. Archived from the original on 30 June 2014. Retrieved 27 July 2014.
  84. "Russian fast reactor reaches full power". Archived from the original on 27 October 2017. Retrieved 27 October 2017.
  85. "До 2030 в России намечено строительство трёх энергоблоков с реакторами БН-1200". AtomInfo.ru. Archived from the original on 5 August 2014. Retrieved 27 July 2014.
  86. "Russia postpones BN-1200 in order to improve fuel design". World Nuclear News. 16 April 2015. Archived from the original on 21 June 2015. Retrieved 19 April 2015.
  87. "Fast moves for nuclear development in Siberia". World Nuclear Association. Archived from the original on 12 October 2012. Retrieved 8 October 2012.
  88. "Department of Energy – Generation IV International Forum Signs Agreement to Collaborate on Sodium Cooled Fast Reactors". Archived from the original on 20 April 2008.
  89. "MHI launches fast breeder group". Nuclear Engineering International. Archived from the original on 28 July 2007. Retrieved 13 March 2011.
  90. World Nuclear News (16 September 2010). "French government puts up funds for Astrid". Archived from the original on 14 July 2014. Retrieved 15 June 2012.
  91. "Quatrième génération: vers un nucléaire durable" (PDF) (in French). CEA. Archived (PDF) from the original on 3 June 2012. Retrieved 15 June 2012.
  92. "France drops plans to build sodium-cooled nuclear reactor". Reuters. 30 August 2019. Archived from the original on 24 September 2019. Retrieved 20 November 2019.
  93. "Flibe Energy". Archived from the original on 7 February 2013. Retrieved 29 October 2011.
  94. "Kirk Sorensen has started a Thorium Power company Flibe Energy". The Next Bi Future. 23 May 2011. Archived from the original on 26 October 2011. Retrieved 30 October 2011.
  95. "Live chat: nuclear thorium technologist Kirk Sorensen". Environment Blog. London: The Guardian (UK). 7 September 2001. Archived from the original on 15 July 2014. Retrieved 30 October 2011.
  96. Martin, William T. (27 September 2011). "New Huntsville company to build thorium-based nuclear reactors". Huntsville Newswire. Archived from the original on 6 April 2012. Retrieved 30 October 2011.{{cite web}}: CS1 maint: unfit URL (link)
  97. "Prototype Prism proposed for Savannah River". World Nuclear News. 28 October 2010. Archived from the original on 28 January 2019. Retrieved 4 November 2010.
  98. Connor, Steve (28 October 2011). "New life for old idea that could dissolve our nuclear waste". The Independent. London. Archived from the original on 29 October 2011. Retrieved 30 October 2011.
  99. "TR10: Traveling Wave Reactor". Technology Review. March 2009. Archived from the original on 4 May 2012. Retrieved 6 March 2009.